Optical Enhancement of Indirect Bandgap 2D Transition Metal Dichalcogenides for Multi‐Functional Optoelectronic Sensors

Author:

Dutta Riya1,Bala Arindam1,Sen Anamika1,Spinazze Michael Ross2,Park Heekyeong1,Choi Woong3,Yoon Youngki2,Kim Sunkook1ORCID

Affiliation:

1. School of Advanced Materials Science and Engineering Sungkyunkwan University Suwon Gyeonggi‐do 16419 Republic of Korea

2. Waterloo Institute for Nanotechnology and the Department of Electrical and Computer Engineering University of Waterloo Waterloo Ontario N2L 3G1 Canada

3. School of Materials Science & Engineering Kookmin University Seoul 02707 Republic of Korea

Abstract

AbstractThe unique electrical and optical properties of transition metal dichalcogenides (TMDs) make them attractive nanomaterials for optoelectronic applications, especially optical sensors. However, the optical characteristics of these materials are dependent on the number of layers. Monolayer TMDs have a direct bandgap that provides higher photoresponsivity compared to multilayer TMDs with an indirect bandgap. Nevertheless, multilayer TMDs are more appropriate for various photodetection applications due to their high carrier density, broad spectral response from UV to near‐infrared, and ease of large‐scale synthesis. Therefore, this review focuses on the modification of the optical properties of devices based on indirect bandgap TMDs and their emerging applications. Several successful developments in optical devices are examined, including band structure engineering, device structure optimization, and heterostructures. Furthermore, it introduces cutting‐edge techniques and future directions for optoelectronic devices based on multilayer TMDs.

Funder

Natural Sciences and Engineering Research Council of Canada

National Research Foundation of Korea

Publisher

Wiley

Subject

Mechanical Engineering,Mechanics of Materials,General Materials Science

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