Super-resolution electron ptychography of low dimensional materials at 30 keV: Beyond the detector limit

Author:

Allen C. S.12ORCID,Danaie M.2ORCID,Warner J. H.34ORCID,Batey D. J.5ORCID,Kirkland A. I.126ORCID

Affiliation:

1. Department of Materials, University of Oxford 1 , Oxford OX1 3PH, United Kingdom

2. Electron Physical Science Imaging Centre, Diamond Light Source Ltd 2 , Didcot OX11 0DE, United Kingdom

3. Materials Science and Engineering Program, Texas Materials Institute, The University of Texas at Austin 3 , Austin, Texas 78712, USA

4. Department of Mechanical Engineering, The University of Texas at Austin 4 Walker , Austin, Texas 78712, USA

5. Diamond Light Source Ltd. 5 , Didcot OX11 0DE, United Kingdom

6. Rosalind Franklin Institute, Harwell Campus 6 , Didcot OX11 0QX, United Kingdom

Abstract

We demonstrate that electron ptychographic phase reconstruction can recover spatial frequencies higher than those directly recorded in the experimental electron diffraction patterns. This ability to recover high angle information from the oversampled low angle information allows an annular detector to be inserted which partially shadows a lower pixelated detector to simultaneously record a conventional annular dark field image and a ptychographic dataset. We apply this approach to 30 keV imaging of monolayer molybdenum disulfide and achieve an Abbe limited resolution of 1.2 ± 0.1Å in our reconstructions.

Funder

Diamond Light Source

Publisher

AIP Publishing

Subject

Physics and Astronomy (miscellaneous)

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