Optimizing the Isoprene Emission Model MEGAN With Satellite and Ground‐Based Observational Constraints

Author:

DiMaria Christian A.1ORCID,Jones Dylan B. A.1ORCID,Worden Helen2ORCID,Bloom A. Anthony3ORCID,Bowman Kevin3ORCID,Stavrakou Trissevgeni4ORCID,Miyazaki Kazuyuki3ORCID,Worden John3ORCID,Guenther Alex5ORCID,Sarkar Chinmoy5ORCID,Seco Roger6ORCID,Park Jeong‐Hoo7,Tota Julio8,Alves Eliane Gomes9ORCID,Ferracci Valerio10ORCID

Affiliation:

1. Department of Physics University of Toronto Toronto ON Canada

2. Atmospheric Chemistry Observations & Modeling Laboratory National Center for Atmospheric Research Boulder CO USA

3. Jet Propulsion Laboratory California Institute of Technology Pasadena CA USA

4. Royal Belgian Institute for Space Aeronomy (BIRA‐IASB) Brussels Belgium

5. Department of Earth System Science University of California Irvine CA USA

6. Institute of Environmental Assessment and Water Research (IDAEA‐CSIC) Barcelona Spain

7. Air Quality Research Division National Institute of Environmental Research Incheon Republic of Korea

8. Julio Tota Instituto de engenharia e Geociências Universidade Federal do Oeste do Pará UFOPA Santarém Brazil

9. Department of Biogeochemical Processes Max Planck Institute for Biogeochemistry Jena Germany

10. School of Water, Energy and Environment Cranfield University Cranfield UK

Abstract

AbstractIsoprene is a hydrocarbon emitted in large quantities by terrestrial vegetation. It is a precursor to several air quality and climate pollutants including ozone. Emission rates vary with plant species and environmental conditions. This variability can be modeled using the Model of Emissions of Gases and Aerosols from Nature (MEGAN). MEGAN parameterizes isoprene emission rates as a vegetation‐specific standard rate which is modulated by scaling factors that depend on meteorological and environmental driving variables. Recent experiments have identified large uncertainties in the MEGAN temperature response parameterization, while the emission rates under standard conditions are poorly constrained in some regions due to a lack of representative measurements and uncertainties in landcover. In this study, we use Bayesian model‐data fusion to optimize the MEGAN temperature response and standard emission rates using satellite‐ and ground‐based observational constraints. Optimization of the standard emission rate with satellite constraints reduced model biases but was highly sensitive to model input errors and drought stress and was found to be inconsistent with ground‐based constraints at an Amazonian field site, reflecting large uncertainties in the satellite‐based emissions. Optimization of the temperature response with ground‐based constraints increased the temperature sensitivity of the model by a factor of five at an Amazonian field site but had no impact at a UK field site, demonstrating significant ecosystem‐dependent variability of the isoprene emission temperature sensitivity. Ground‐based measurements of isoprene across a wide range of ecosystems will be key for obtaining an accurate representation of isoprene emission temperature sensitivity in global biogeochemical models.

Funder

Natural Sciences and Engineering Research Council of Canada

Publisher

American Geophysical Union (AGU)

Subject

Space and Planetary Science,Earth and Planetary Sciences (miscellaneous),Atmospheric Science,Geophysics

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