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Kinetics of the reactions of NO3 radical with alkanes

Published:2019 Issue:8 Volume:21 Page:4246-4257
ISSN:1463-9076
Container-title:Physical Chemistry Chemical Physics
language:en
Short-container-title:Phys. Chem. Chem. Phys.

Author:

Zhou Li¹²³⁴⁵,Ravishankara A. R.¹²³⁴⁵^ORCID,Brown Steven S.⁶⁷⁸⁹¹⁰^ORCID,Zarzana Kyle J.⁶⁷⁸¹¹¹⁰^ORCID,Idir Mahmoud¹²³⁴⁵,Daële Véronique¹²³⁴⁵,Mellouki Abdelwahid¹²³⁴⁵^ORCID

Affiliation:

1. Institut de Combustion

2. Aérothermique

3. Réactivité et Environnement/OSUC

4. CNRS

5. 45071 Orléans Cedex 02

6. NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division

7. Boulder

8. USA

9. Department of Chemistry

10. University of Colorado Boulder

11. Cooperative Institute for Research in Environmental Sciences

Abstract

The rate coefficients for the reactions of NO₃ radicals with methane (CH₄), ethane (C₂H₆), propane (C₃H₈), n-butane (n-C₄H₁₀), iso-butane (iso-C₄H₁₀), 2,3-dimethylbutane (C₆H₁₄), cyclopentane (C₅H₁₀) and cyclohexane (C₆H₁₂) at atmosphere pressure (1000 ± 5 hPa) and room temperature (298 ± 1.5 K) were measured using an absolute method.

Funder

Centre National de la Recherche Scientifique

Agence Nationale de la Recherche

Horizon 2020 Framework Programme

National Oceanic and Atmospheric Administration

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

Link

http://pubs.rsc.org/en/content/articlepdf/2019/CP/C8CP07675H

Reference37 articles.

1. Reactive nitrogen partitioning and its relationship to winter ozone events in Utah

2. Kinetics of the gas-phase reactions of nitrate (NO3) radicals with a series of alkanes at 296 .+-. 2 K

3. Rate constants for the gas-phase reactions of the nitrate radical with a series of organic compounds at 296 .+-. 2 K

4. Temperature dependence of reactions of the nitrate radical with alkanes

5. Use of a stopped-flow technique to measure the rate constants at room temperature for reactions between the nitrate radical and various organic species

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