Absolute determination of chemical kinetic rate constants by optical tracking the reaction on the second timescale using cavity-enhanced absorption spectroscopy

Author:

Yi Hongming1ORCID,Meng Lingshuo12,Wu Tao3,Lauraguais Amélie1,Coeur Cecile1,Tomas Alexandre2ORCID,Fu Hongbo4,Gao Xiaoming5,Chen Weidong1

Affiliation:

1. Laboratoire de Physicochimie de l’Atmosphère, Université du Littoral Côte d’Opale, 59140 Dunkerque, France

2. IMT Nord Europe, Institut Mines-Télécom, Univ. Lille, Center for Energy and Environment, 59000 Lille, France

3. Key Laboratory of Nondestructive Test, Nanchang Hangkong University, Nanchang 330063, China

4. Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Institute of Atmospheric Sciences, Fudan University, Shanghai, 200433, China

5. Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China

Abstract

We report a new spectroscopic platform coupled to an atmospheric simulation chamber for the direct determination of chemical rate constants with high accuracy at a second time-scale resolution.

Funder

Agence Nationale de la Recherche

LABoratoires d’EXcellence ARCANE

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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