Design of Electrostatic Aberration Correctors for Scanning Transmission Electron Microscopy

Author:

Ribet Stephanie M123ORCID,Zeltmann Steven E45,Bustillo Karen C3,Dhall Rohan3,Denes Peter6,Minor Andrew M35,dos Reis Roberto127ORCID,Dravid Vinayak P127ORCID,Ophus Colin3

Affiliation:

1. Department of Materials Science and Engineering, Northwestern University , Evanston, IL 60208 , USA

2. International Institute of Nanotechnology, Northwestern University , Evanston, IL 60208 , USA

3. National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Laboratory , Berkeley, CA 94720 , USA

4. Platform for the Accelerated Realization, Analysis, and Discovery of Interface Materials (PARADIM), Cornell University , Ithaca, NY 14853 , USA

5. Department of Materials Science and Engineering, University of California, Berkeley , Berkeley, CA 94720 , USA

6. Molecular Foundry, Lawrence Berkeley National Laboratory , Berkeley, CA 94720 , USA

7. The NUANCE Center, Northwestern University , Evanston, IL 60208 , USA

Abstract

Abstract In a scanning transmission electron microscope (STEM), producing a high-resolution image generally requires an electron beam focused to the smallest point possible. However, the magnetic lenses used to focus the beam are unavoidably imperfect, introducing aberrations that limit resolution. Modern STEMs overcome this by using hardware aberration correctors comprised of many multipole elements, but these devices are complex, expensive, and can be difficult to tune. We demonstrate a design for an electrostatic phase plate that can act as an aberration corrector. The corrector is comprised of annular segments, each of which is an independent two-terminal device that can apply a constant or ramped phase shift to a portion of the electron beam. We show the improvement in image resolution using an electrostatic corrector. Engineering criteria impose that much of the beam within the probe-forming aperture be blocked by support bars, leading to large probe tails for the corrected probe that sample the specimen beyond the central lobe. We also show how this device can be used to create other STEM beam profiles such as vortex beams and probes with a high degree of phase diversity, which improve information transfer in ptychographic reconstructions.

Funder

U.S. Department of Energy

Office of Science

Workforce Development for Teachers and Scientists

Office of Science Graduate Student Research (SCGSR) program

Oak Ridge Institute for Science and Education

National Science Foundation

US Department of Energy Early Career Research Program

SHyNE Resource

International Institute of Nanotechnology

Northwestern’s MRSEC program

Basic Energy Sciences

Publisher

Oxford University Press (OUP)

Subject

Instrumentation

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