The role of methane in projections of 21st century stratospheric water vapour
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Published:2016-10-21
Issue:20
Volume:16
Page:13067-13080
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ISSN:1680-7324
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Container-title:Atmospheric Chemistry and Physics
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language:en
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Short-container-title:Atmos. Chem. Phys.
Author:
Revell Laura E.ORCID, Stenke AndreaORCID, Rozanov EugeneORCID, Ball WilliamORCID, Lossow StefanORCID, Peter Thomas
Abstract
Abstract. Stratospheric water vapour (SWV) is an important component of the Earth's atmosphere as it affects both radiative balance and the chemistry of the atmosphere. Key processes driving changes in SWV include dehydration of air masses transiting the cold-point tropopause (CPT) and methane oxidation. We use a chemistry–climate model to simulate changes in SWV through the 21st century following the four canonical representative concentration pathways (RCPs). Furthermore, we quantify the contribution that methane oxidation makes to SWV following each of the RCPs. Although the methane contribution to SWV maximizes in the upper stratosphere, modelled SWV trends are found to be driven predominantly by warming of the CPT rather than by increasing methane oxidation. SWV changes by −5 to 60 % (depending on the location in the atmosphere and emissions scenario) and increases in the lower stratosphere in all RCPs through the 21st century. Because the lower stratosphere is where water vapour radiative forcing maximizes, SWV's influence on surface climate is also expected to increase through the 21st century.
Publisher
Copernicus GmbH
Subject
Atmospheric Science
Reference65 articles.
1. Arfeuille, F., Luo, B. P., Heckendorn, P., Weisenstein, D., Sheng, J. X., Rozanov, E., Schraner, M., Brönnimann, S., Thomason, L. W., and Peter, T.: Modeling the stratospheric warming following the Mt. Pinatubo eruption: uncertainties in aerosol extinctions, Atmos. Chem. Phys., 13, 11221–11234, https://doi.org/10.5194/acp-13-11221-2013, 2013. 2. Austin, J., Wilson, J., and Li, F.: Evolution of water vapor concentrations and stratospheric age of air in coupled chemistry-climate model simulations, J. Atmos. Sci., 64, 905–921, https://doi.org/10.1175/JAS3866.1, 2007. 3. Bates, D. R. and Nicolet, M.: Atmospheric hydrogen, Publ. Astron. Soc. Pac., 62, 106–110, 1950. 4. Bekki, S., Rap, A., Poulain, V., Dhomse, S., Marchand, M., Lefevre, F., Forster, P. M., Szopa, S., and Chipperfield, M. P.: Climate impact of stratospheric ozone recovery, Geophys. Res. Lett., 40, 2796–2800, https://doi.org/10.1002/grl.50358, 2013. 5. Brasseur, G. and Solomon, S.: Composition and Chemistry, in: Aeronomy of the Middle Atmosphere, 3rd Edn., Springer, Dordrecht, Netherlands, 265–422, 2005.
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