Upper tropospheric CH<sub>4</sub> and CO affected by the South Asian summer monsoon during the Oxidation Mechanism Observations mission
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Published:2019-02-13
Issue:3
Volume:19
Page:1915-1939
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ISSN:1680-7324
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Container-title:Atmospheric Chemistry and Physics
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language:en
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Short-container-title:Atmos. Chem. Phys.
Author:
Tomsche Laura, Pozzer AndreaORCID, Ojha NarendraORCID, Parchatka Uwe, Lelieveld JosORCID, Fischer Horst
Abstract
Abstract. The Asian monsoon anticyclone (AMA) is annual phenomenon in the
northern hemispheric upper troposphere and lower stratosphere. It is part of
the South Asian summer monsoon system, and it has a clearly observable
signature due to the vertical transport of polluted air masses from the surface
to the upper troposphere by monsoon convection. We performed in situ
measurements of carbon monoxide (CO) and methane (CH4) in the region of
monsoon outflow and in background air in the upper troposphere
(Mediterranean, Arabian Peninsula, and Arabian Sea) using optical absorption
spectroscopy on board the High Altitude and LOng range (HALO) research
aircraft during the OMO (Oxidation Mechanism Observations) mission in summer
2015. We identified the transport pathways and the origin of the trace gases
with back trajectories, which were calculated using the Lagrangian particle dispersion
model FLEXPART, and we compared the in situ data with simulations of the
atmospheric chemistry general circulation model EMAC. CH4 and CO mixing
ratios were found to be enhanced within the AMA, the in situ data increased
by 72.1 and 20.1 ppbv on average, respectively, and originated in the South
Asian region (Indo-Gangetic Plain, northeastern India, Bangladesh, and the Bay of
Bengal). It appears that CH4 is an ideal monsoon tracer in the upper
troposphere due to its extended lifetime and the strong South Asian
emissions. Furthermore, we used the measurements and model results to study
the dynamics of the AMA over several weeks during the monsoon season, with an
emphasis on the southern and western areas in the upper troposphere. We
distinguished four AMA modes based on different meteorological conditions.
On one occasion we observed that under the influence of dwindling flow
the transport barrier between the anticyclone and its surroundings weakened,
expelling air masses from the AMA. The trace gases exhibited a distinct
AMA fingerprint; we also found that CH4 accumulated over the
course of the OMO campaign.
Publisher
Copernicus GmbH
Subject
Atmospheric Science
Reference67 articles.
1. Baker, A. K., Schuck, T. J., Brenninkmeijer, C. A., Rauthe-Schöch, A.,
Slemr, F., Velthoven, P. F., and Lelieveld, J.: Estimating the contribution
of monsoon-related biogenic production to methane emissions from South Asia
using CARIBIC observations, Geophys. Res. Lett., 39, L10813, https://doi.org/10.1029/2012gl051756, 2012. 2. Barret, B., Sauvage, B., Bennouna, Y., and Le Flochmoen, E.:
Upper-tropospheric CO and O3 budget during the Asian summer monsoon, Atmos.
Chem. Phys., 16, 9129–9147, https://doi.org/10.5194/acp-16-9129-2016, 2016. 3. Bergamaschi, P., Houweling, S., Segers, A., Krol, M., Frankenberg, C.,
Scheepmaker, R., Dlugokencky, E., Wofsy, S., Kort, E., and Sweeney, C.:
Atmospheric CH4 in the first decade of the 21st century: Inverse modeling
analysis using SCIAMACHY satellite retrievals and NOAA surface measurements,
J. Geophys. Res.-Atmos., 118, 7350–7369, 2013. 4. Bergman, J. W., Fierli, F., Jensen, E. J., Honomichl, S., and Pan, L. L.:
Boundary layer sources for the Asian anticyclone: Regional contributions to
a vertical conduit, J. Geophys. Res.-Atmos., 118,
2560–2575, 2013. 5. Bloom, A. A., Bowman, K. W., Lee, M., Turner, A. J., Schroeder, R., Worden,
J. R., Weidner, R., McDonald, K. C., and Jacob, D. J.: A global wetland
methane emissions and uncertainty dataset for atmospheric chemical transport
models (WetCHARTs version 1.0), Geosci. Model Dev., 10, 2141–2156,
https://doi.org/10.5194/gmd-10-2141-2017, 2017.
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