The long-term transport and radiative impacts of the 2017 British Columbia pyrocumulonimbus smoke aerosols in the stratosphere
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Published:2021-08-12
Issue:15
Volume:21
Page:12069-12090
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ISSN:1680-7324
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Container-title:Atmospheric Chemistry and Physics
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language:en
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Short-container-title:Atmos. Chem. Phys.
Author:
Das SampaORCID, Colarco Peter R.ORCID, Oman Luke D., Taha GhassanORCID, Torres Omar
Abstract
Abstract. Interactions of meteorology with wildfires in British Columbia,
Canada, during August 2017 led to three major pyrocumulonimbus (pyroCb)
events that resulted in the injection of large amounts of smoke aerosols and
other combustion products at the local upper troposphere and lower
stratosphere (UTLS). These plumes of UTLS smoke with elevated values of
aerosol extinction and backscatter compared to the background state were
readily tracked by multiple satellite-based instruments as they spread
across the Northern Hemisphere (NH). The plumes were observed in the lower
stratosphere for about 8–10 months following the fire injections, with a
stratospheric aerosol e-folding time of about 5 months. To investigate the
radiative impacts of these events on the Earth system, we performed a number
of simulations with the Goddard Earth Observing System (GEOS) atmospheric
general circulation model (AGCM). Observations from multiple remote-sensing
instruments were used to calibrate the injection parameters (location,
amount, composition and heights) and optical properties of the smoke
aerosols in the model. The resulting simulations of three-dimensional smoke
transport were evaluated for a year from the day of injections using daily
observations from OMPS-LP (Ozone Mapping Profiler Suite Limb Profiler). The
model-simulated rate of ascent, hemispheric spread and residence time (or
e-folding time) of the smoke aerosols in the stratosphere are in close
agreement with OMPS-LP observations. We found that both aerosol self-lofting
and the large-scale atmospheric motion play important roles in lifting the
smoke plumes from near the tropopause altitudes (∼ 12 km) to
about 22–23 km into the atmosphere. Further, our estimations of the
radiative impacts of the pyroCb-emitted smoke aerosols showed that the smoke
caused an additional warming of the atmosphere by about 0.6–1 W/m2
(zonal mean) that persisted for about 2–3 months after the injections in
regions north of 40∘ N. The surface experienced a comparable magnitude
of cooling. The atmospheric warming is mainly located in the stratosphere,
coincident with the location of the smoke plumes, leading to an increase in
zonal mean shortwave (SW) heating rates of 0.02–0.04 K/d during September
2017.
Funder
Earth Sciences Division
Publisher
Copernicus GmbH
Subject
Atmospheric Science
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