Assessing the ability to derive rates of polar middle-atmospheric descent using trace gas measurements from remote sensors
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Published:2018-02-02
Issue:3
Volume:18
Page:1457-1474
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ISSN:1680-7324
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Container-title:Atmospheric Chemistry and Physics
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language:en
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Short-container-title:Atmos. Chem. Phys.
Author:
Ryan Niall J., Kinnison Douglas E., Garcia Rolando R.ORCID, Hoffmann Christoph G.ORCID, Palm MathiasORCID, Raffalski UweORCID, Notholt Justus
Abstract
Abstract. We investigate the reliability of using trace gas
measurements from remote sensing instruments to infer polar atmospheric
descent rates during winter within 46–86 km altitude. Using output from
the Specified Dynamics Whole Atmosphere Community Climate Model (SD-WACCM)
between 2008 and 2014, tendencies of carbon monoxide (CO) volume mixing
ratios (VMRs) are used to assess a common assumption of dominant vertical
advection of tracers during polar winter. The results show that dynamical
processes other than vertical advection are not negligible, meaning that the
transport rates derived from trace gas measurements do not represent the
mean descent of the atmosphere. The relative importance of vertical
advection is lessened, and exceeded by other processes, during periods
directly before and after a sudden stratospheric warming, mainly due to an
increase in eddy transport. It was also found that CO chemistry cannot be
ignored in the mesosphere due to the night-time layer of OH at approximately
80 km altitude. CO VMR profiles from the Kiruna Microwave Radiometer and the
Microwave Limb Sounder were compared to SD-WACCM output, and show good
agreement on daily and seasonal timescales. SD-WACCM CO profiles are
combined with the CO tendencies to estimate errors involved in calculating
the mean descent of the atmosphere from remote sensing measurements. The
results indicate errors on the same scale as the calculated descent rates,
and that the method is prone to a misinterpretation of the direction of air
motion. The “true” rate of atmospheric descent is seen to be masked by
processes, other than vertical advection, that affect CO. We suggest an
alternative definition of the rate calculated using remote sensing
measurements: not as the mean descent of the atmosphere, but as an effective
rate of vertical transport for the trace gas under observation.
Funder
Universität Bremen Bundesministerium für Bildung und Forschung
Publisher
Copernicus GmbH
Subject
Atmospheric Science
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