Simulation model of Reactive Nitrogen Species in an Urban Atmosphere using a Deep Neural Network: RNDv1.0
-
Published:2023-09-13
Issue:17
Volume:16
Page:5251-5263
-
ISSN:1991-9603
-
Container-title:Geoscientific Model Development
-
language:en
-
Short-container-title:Geosci. Model Dev.
Author:
Gil JunsuORCID, Lee MeehyeORCID, Kim Jeonghwan, Lee Gangwoong, Ahn Joonyoung, Kim Cheol-HeeORCID
Abstract
Abstract. Nitrous acid (HONO) plays an important role in the
formation of ozone and fine aerosols in the urban atmosphere. In this study,
a new simulation approach is presented to calculate the HONO mixing ratios
using a deep neural technique based on measured variables. The Reactive
Nitrogen Species using a Deep Neural Network (RND) simulation is implemented
in Python. The first version of RND (RNDv1.0) is trained, validated, and
tested with HONO measurement data obtained in Seoul, South Korea, from 2016 to 2021.
RNDv1.0 is constructed using k-fold cross validation and evaluated with
index of agreement, correlation coefficient, root mean squared error, and
mean absolute error. The results show that RNDv1.0 adequately represents the
main characteristics of the measured HONO, and it is thus proposed as a
supplementary model for calculating the HONO mixing ratio in a polluted
urban environment.
Funder
National Research Foundation of Korea Korea Institute of Science and Technology
Publisher
Copernicus GmbH
Reference70 articles.
1. Akimoto, H. and Tanimoto, H.: Review of Comprehensive Measurements of
Speciated NOy and its Chemistry: Need for Quantifying the Role of
Heterogeneous Processes of HNO3 and HONO, Aerosol Air Qual. Res., 21, 200395, https://doi.org/10.4209/aaqr.2020.07.0395,
2021. 2. Akimoto, H., Nagashima, T., Li, J., Fu, J. S., Ji, D., Tan, J., and Wang, Z.: Comparison of surface ozone simulation among selected regional models in MICS-Asia III – effects of chemistry and vertical transport for the causes of difference, Atmos. Chem. Phys., 19, 603–615, https://doi.org/10.5194/acp-19-603-2019, 2019. 3. Anderson, D. C., Loughner, C. P., Diskin, G., Weinheimer, A., Canty, T. P.,
Salawitch, R. J., Worden, H. M., Fried, A., Mikoviny, T., and Wisthaler, A.:
Measured and modeled CO and NOy in DISCOVER-AQ: An evaluation of emissions
and chemistry over the eastern US, Atmos. Environ., 96, 78–87, 2014. 4. Appel, K. W., Bash, J. O., Fahey, K. M., Foley, K. M., Gilliam, R. C., Hogrefe, C., Hutzell, W. T., Kang, D., Mathur, R., Murphy, B. N., Napelenok, S. L., Nolte, C. G., Pleim, J. E., Pouliot, G. A., Pye, H. O. T., Ran, L., Roselle, S. J., Sarwar, G., Schwede, D. B., Sidi, F. I., Spero, T. L., and Wong, D. C.: The Community Multiscale Air Quality (CMAQ) model versions 5.3 and 5.3.1: system updates and evaluation, Geosci. Model Dev., 14, 2867–2897, https://doi.org/10.5194/gmd-14-2867-2021, 2021. 5. Arcomano, T., Szunyogh, I., Wikner, A., Pathak, J., Hunt, B. R., and Ott,
E.: A Hybrid Approach to Atmospheric Modeling that Combines Machine Learning
with a Physics-Based Numerical Model, J. Adv. Model. Earth Sy., 14, e2021MS002712, https://doi.org/10.1029/2021MS002712,
2021.
Cited by
1 articles.
订阅此论文施引文献
订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献
|
|