Simulation model of Reactive Nitrogen Species in an Urban Atmosphere using a Deep Neural Network: RNDv1.0

Author:

Gil JunsuORCID,Lee MeehyeORCID,Kim Jeonghwan,Lee Gangwoong,Ahn Joonyoung,Kim Cheol-HeeORCID

Abstract

Abstract. Nitrous acid (HONO) plays an important role in the formation of ozone and fine aerosols in the urban atmosphere. In this study, a new simulation approach is presented to calculate the HONO mixing ratios using a deep neural technique based on measured variables. The Reactive Nitrogen Species using a Deep Neural Network (RND) simulation is implemented in Python. The first version of RND (RNDv1.0) is trained, validated, and tested with HONO measurement data obtained in Seoul, South Korea, from 2016 to 2021. RNDv1.0 is constructed using k-fold cross validation and evaluated with index of agreement, correlation coefficient, root mean squared error, and mean absolute error. The results show that RNDv1.0 adequately represents the main characteristics of the measured HONO, and it is thus proposed as a supplementary model for calculating the HONO mixing ratio in a polluted urban environment.

Funder

National Research Foundation of Korea

Korea Institute of Science and Technology

Publisher

Copernicus GmbH

Subject

General Medicine

Reference70 articles.

1. Akimoto, H. and Tanimoto, H.: Review of Comprehensive Measurements of Speciated NOy and its Chemistry: Need for Quantifying the Role of Heterogeneous Processes of HNO3 and HONO, Aerosol Air Qual. Res., 21, 200395, https://doi.org/10.4209/aaqr.2020.07.0395, 2021.

2. Akimoto, H., Nagashima, T., Li, J., Fu, J. S., Ji, D., Tan, J., and Wang, Z.: Comparison of surface ozone simulation among selected regional models in MICS-Asia III – effects of chemistry and vertical transport for the causes of difference, Atmos. Chem. Phys., 19, 603–615, https://doi.org/10.5194/acp-19-603-2019, 2019.

3. Anderson, D. C., Loughner, C. P., Diskin, G., Weinheimer, A., Canty, T. P., Salawitch, R. J., Worden, H. M., Fried, A., Mikoviny, T., and Wisthaler, A.: Measured and modeled CO and NOy in DISCOVER-AQ: An evaluation of emissions and chemistry over the eastern US, Atmos. Environ., 96, 78–87, 2014.

4. Appel, K. W., Bash, J. O., Fahey, K. M., Foley, K. M., Gilliam, R. C., Hogrefe, C., Hutzell, W. T., Kang, D., Mathur, R., Murphy, B. N., Napelenok, S. L., Nolte, C. G., Pleim, J. E., Pouliot, G. A., Pye, H. O. T., Ran, L., Roselle, S. J., Sarwar, G., Schwede, D. B., Sidi, F. I., Spero, T. L., and Wong, D. C.: The Community Multiscale Air Quality (CMAQ) model versions 5.3 and 5.3.1: system updates and evaluation, Geosci. Model Dev., 14, 2867–2897, https://doi.org/10.5194/gmd-14-2867-2021, 2021.

5. Arcomano, T., Szunyogh, I., Wikner, A., Pathak, J., Hunt, B. R., and Ott, E.: A Hybrid Approach to Atmospheric Modeling that Combines Machine Learning with a Physics-Based Numerical Model, J. Adv. Model. Earth Sy., 14, e2021MS002712, https://doi.org/10.1029/2021MS002712, 2021.

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