East Asian methane emissions inferred from high-resolution inversions of GOSAT and TROPOMI observations: a comparative and evaluative analysis
-
Published:2023-07-19
Issue:14
Volume:23
Page:8039-8057
-
ISSN:1680-7324
-
Container-title:Atmospheric Chemistry and Physics
-
language:en
-
Short-container-title:Atmos. Chem. Phys.
Author:
Liang RuosiORCID, Zhang YuzhongORCID, Chen Wei, Zhang Peixuan, Liu Jingran, Chen Cuihong, Mao Huiqin, Shen GuofengORCID, Qu ZhenORCID, Chen Zichong, Zhou MinqiangORCID, Wang Pucai, Parker Robert J.ORCID, Boesch Hartmut, Lorente AlbaORCID, Maasakkers Joannes D.ORCID, Aben Ilse
Abstract
Abstract. We apply atmospheric methane column retrievals from two
different satellite instruments (Greenhouse gases Observing SATellite – GOSAT; TROPOspheric Monitoring Instrument – TROPOMI) to a regional inversion
framework to quantify East Asian methane emissions for 2019 at
0.5∘ × 0.625∘ horizontal resolution. The goal
is to assess if GOSAT (relatively mature but sparse) and TROPOMI (new and
dense) observations inform consistent methane emissions from East Asia with
identically configured inversions. Comparison of the results from the two
inversions shows similar correction patterns to the prior inventory in
central northern China, central southern China, northeastern China, and Bangladesh,
with less than 2.6 Tg a−1 differences in regional posterior emissions.
The two inversions, however, disagree over some important regions,
particularly in northern India and eastern China. The methane emissions
inferred from GOSAT observations are 7.7 Tg a−1 higher than those from
TROPOMI observations over northern India but 6.4 Tg a−1 lower over eastern
China. The discrepancies between the two inversions are robust against
varied inversion configurations (i.e., assimilation window and error
specifications). We find that the lower methane emissions from eastern China
inferred by the GOSAT inversion are more consistent with independent
ground-based in situ and total column (TCCON) observations, indicating that the
TROPOMI retrievals may have high XCH4 biases in this region. We also
evaluate inversion results against tropospheric aircraft observations over
India during 2012–2014 by using a consistent GOSAT inversion of earlier
years as an intercomparison platform. This indirect evaluation favors lower
methane emissions from northern India inferred by the TROPOMI inversion. We
find that in this case the discrepancy in emission inference is contributed
by differences in data coverage (almost no observations by GOSAT vs. good
spatial coverage by TROPOMI) over the Indo-Gangetic Plain. The two
inversions also differ substantially in their posterior estimates for
northwestern China and neighboring Kazakhstan, which is mainly due to
seasonally varying biases between GOSAT and TROPOMI XCH4 data that
correlate with changes in surface albedo.
Funder
National Key Research and Development Program of China National Natural Science Foundation of China
Publisher
Copernicus GmbH
Subject
Atmospheric Science
Reference80 articles.
1. Alexe, M., Bergamaschi, P., Segers, A., Detmers, R., Butz, A., Hasekamp, O., Guerlet, S., Parker, R., Boesch, H., Frankenberg, C., Scheepmaker, R. A., Dlugokencky, E., Sweeney, C., Wofsy, S. C., and Kort, E. A.: Inverse modelling of CH4 emissions for 2010–2011 using different satellite retrieval products from GOSAT and SCIAMACHY, Atmos. Chem. Phys., 15, 113–133, https://doi.org/10.5194/acp-15-113-2015, 2015. 2. Bloom, A. A., Bowman, K. W., Lee, M., Turner, A. J., Schroeder, R., Worden, J. R., Weidner, R., McDonald, K. C., and Jacob, D. J.: A global wetland methane emissions and uncertainty dataset for atmospheric chemical transport models (WetCHARTs version 1.0), Geosci. Model Dev., 10, 2141–2156, https://doi.org/10.5194/gmd-10-2141-2017, 2017. 3. Brasseur, G. P. and Jacob, D. J.: Modeling of Atmospheric Chemistry,
Cambridge University Press, Cambridge, USA, https://doi.org/10.1017/9781316544754, 2017. 4. Butz, A., Guerlet, S., Hasekamp, O. P., Schepers, D., Galli, A., Aben, I.,
Frankenberg, C., Hartmann, J.-M., Tran, H., Kuze, A., Keppel-Aleks, G.,
Toon, G. C., Wunch, D., Wennberg, P. O., Deutscher, N. M., Griffith, D. W.
T., Macatangay, R., Messerschmidt, J., Notholt, J., and Warneke, T.: Toward
accurate CO2 and CH4 observations from GOSAT, Geophys. Res. Lett., 38,
L14812, https://doi.org/10.1029/2011GL047888, 2011. 5. Chen, Z., Jacob, D. J., Nesser, H., Sulprizio, M. P., Lorente, A., Varon, D. J., Lu, X., Shen, L., Qu, Z., Penn, E., and Yu, X.: Methane emissions from China: a high-resolution inversion of TROPOMI satellite observations, Atmos. Chem. Phys., 22, 10809–10826, https://doi.org/10.5194/acp-22-10809-2022, 2022.
Cited by
3 articles.
订阅此论文施引文献
订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献
|
|