Evaluation of regional background particulate matter concentration based on vertical distribution characteristics
-
Published:2015-10-07
Issue:19
Volume:15
Page:11165-11177
-
ISSN:1680-7324
-
Container-title:Atmospheric Chemistry and Physics
-
language:en
-
Short-container-title:Atmos. Chem. Phys.
Author:
Han S.,Zhang Y.,Wu J.,Zhang X.,Tian Y.,Wang Y.,Ding J.,Yan W.,Bi X.,Shi G.,Cai Z.,Yao Q.,Huang H.,Feng Y.
Abstract
Abstract. Heavy regional particulate matter (PM) pollution in China has resulted in an important and urgent need for joint control actions among cities. It is advisable to improve the understanding of the regional background concentration of PM for the development of efficient and effective joint control policies. With the increase of height the influence of source emission on local air quality decreases with altitude, but the characteristics of regional pollution gradually become obvious. A method to estimate regional background PM concentration is proposed in this paper, based on the vertical characteristics of periodic variation in the atmospheric boundary layer structure and particle mass concentration, as well as the vertical distribution of particle size, chemical composition and pollution source apportionment. According to the method, the averaged regional background PM2.5 concentration in July, August and September 2009, being extracted from the original time series in Tianjin, was 40 ± 20, 64 ± 17 and 53 ± 11 μg m−3, respectively.
Funder
National Natural Science Foundation of China
Publisher
Copernicus GmbH
Subject
Atmospheric Science
Reference60 articles.
1. Andreae, M. O., Acevedo, O. C., Araùjo, A., Artaxo, P., Barbosa, C. G. G., Barbosa, H. M. J., Brito, J., Carbone, S., Chi, X., Cintra, B. B. L., da Silva, N. F., Dias, N. L., Dias-Júnior, C. Q., Ditas, F., Ditz, R., Godoi, A. F. L., Godoi, R. H. M., Heimann, M., Hoffmann, T., Kesselmeier, J., Könemann, T., Krüger, M. L., Lavric, J. V., Manzi, A. O., Moran-Zuloaga, D., Nölscher, A. C., Santos Nogueira, D., Piedade, M. T. F., Pöhlker, C., Pöschl, U., Rizzo, L. V., Ro, C.-U., Ruckteschler, N., Sá, L. D. A., Sá, M. D. O., Sales, C. B., Santos, R. M. N. D., Saturno, J., Schöngart, J., Sörgel, M., de Souza, C. M., de Souza, R. A. F., Su, H., Targhetta, N., Tóta, J., Trebs, I., Trumbore, S., van Eijck, A., Walter, D., Wang, Z., Weber, B., Williams, J., Winderlich, J., Wittmann, F., Wolff, S., and Yáñez-Serrano, A. M.: The Amazon Tall Tower Observatory (ATTO) in the remote Amazon Basin: overview of first results from ecosystem ecology, meteorology, trace gas, and aerosol measurements, Atmos. Chem. Phys. Discuss., 15, 11599–11726, https://doi.org/10.5194/acpd-15-11599-2015, 2015. 2. Bi, X., Feng, Y., Wu, J., Wang, Y., and Zhu, T.: Source apportionment of PM10 in six cities of northern China, Atmos. Environ., 41, 903–912, 2007. 3. Brown, S. S., Thornton, J. A., Keene, W. C., Pszenny, A. A. P., Sive, B. C., Dubé, W. P., Wagner, N. L., Young, C. J., Riedel, T. P., Roberts, J. M., VandenBoer, T. C., Bahreini, R., Öztürk, F., Middlebrook, A. M., Kim, S., Hübler, G., and Wolfe, D. E.: Nitrogen, Aerosol Composition, and Halogens on a Tall Tower (NACHTT): Overview of a wintertime air chemistry field study in the front range urban corridor of Colorado, J. Geophys. Res., 118, 8067–8085, https://doi.org/10.1002/jgrd.50537, 2013. 4. Cao, J. J., Lee, S. C., Ho, K. F., Zhang, X. Y., Zou, S. C., Fung, K., Chow, J. C., and Watson, J. G.: Characteristics of carbonaceous aerosol in Pearl River Delta Region, China during 2001 winter period, Atmos. Environ., 37, 1451–1460, 2003. 5. Cao, J. J., Tie, X. X., Dabberdt, W. F., Tang, J., Zhao, Z. Z., An, Z. S., Shen, Z. X., and Feng, Y. C.: On the potential high acid deposition in northeastern China, J. Geophys. Res., 118, 4834–4846, https://doi.org/10.1002/jgrd.50381, 2013.
Cited by
46 articles.
订阅此论文施引文献
订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献
|
|