In situ measurements of non-equilibrium positron state defects during He irradiation in Si

Author:

Auguste R.1ORCID,Liedke M. O.2ORCID,Butterling M.2ORCID,Uberuaga B. P.3ORCID,Selim F. A.45ORCID,Wagner A.2ORCID,Hosemann P.167ORCID

Affiliation:

1. Department of Nuclear Engineering, University of California at Berkeley 1 , Berkeley, California 94720, USA

2. Institute of Radiation Physics, Helmholtz-Zentrum Dresden-Rossendorf 2 , Bautzner Landstr. 400, 01328 Dresden, Germany

3. Materials Science and Technology Division, Los Alamos National Laboratory 3 , Los Alamos, New Mexico 87545, USA

4. Center for Photochemical Sciences, Bowling Green State University 4 , Bowling Green, Ohio 43403, USA

5. Department of Physics and Astronomy, Bowling Green State University 5 , Bowling Green, Ohio 43403, USA

6. Lawrence Berkeley National Laboratory, Material Science Division 6 , Berkeley, California 94720, USA

7. Department of Mechanical Engineering, University of California at Berkeley 7 , Berkeley, California 94720, USA

Abstract

Radiation-induced property changes in materials originate from the energy transfer from an incoming particle to the existing lattice, displacing atoms. The displaced atoms can cause the formation of extended defects including dislocation loops, voids, or precipitates. The non-equilibrium defects created during damage events determine the extent of these larger defects and are a function of dose rate, material, and temperature. However, these defects are transient and can only be probed indirectly. This work presents direct experimental measurements and evidence of irradiated non-equilibrium vacancy formation, where in situ positron annihilation spectroscopy was used to prove the generation of non-equilibrium defects in silicon.

Funder

U.S. Department of Energy

Ron & Gail Gester Fellowship

Publisher

AIP Publishing

Subject

General Physics and Astronomy

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