Electronic energy transport in nanoscale Au/Fe hetero-structures in the perspective of ultrafast lattice dynamics

Author:

Mattern M.1,von Reppert A.1ORCID,Zeuschner S. P.12ORCID,Pudell J.-E.2ORCID,Kühne F.3,Diesing D.4ORCID,Herzog M.1ORCID,Bargheer M.12ORCID

Affiliation:

1. Institut für Physik & Astronomie, Universität Potsdam, Karl-Liebknecht-Str. 24-25, 14476 Potsdam, Germany

2. Helmholtz-Zentrum Berlin für Materialien und Energie, Wilhelm-Conrad-Röntgen Campus, BESSY II, Albert-Einstein-Strasse 15, 12489 Berlin, Germany

3. Faculty of Physics and Center for Nanointegration (CENIDE), University of Duisburg-Essen, Lotharstrasse 1, 47057 Duisburg, Germany

4. Faculty of Chemistry, University of Duisburg-Essen, Universitätsstr. 5, 45141 Essen, Germany

Abstract

We study the ultrafast electronic transport of energy in a photoexcited nanoscale Au/Fe hetero-structure by modeling the spatiotemporal profile of energy densities that drives transient strain, which we quantify by femtosecond x-ray diffraction. This flow of energy is relevant for intrinsic demagnetization and ultrafast spin transport. We measured lattice strain for different Fe layer thicknesses ranging from few atomic layers to several nanometers and modeled the spatiotemporal flow of energy densities. The combination of a high electron-phonon coupling coefficient and a large Sommerfeld constant in Fe is found to yield electronic transfer of nearly all energy from Au to Fe within the first hundreds of femtoseconds.

Funder

Deutsche Forschungsgemeinschaft

Publisher

AIP Publishing

Subject

Physics and Astronomy (miscellaneous)

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