Radiative and Chemical Effects of Non‐Homogeneous Methane on Terrestrial Carbon Fluxes in Asia

Author:

Zhang Qian1,Wang Tijian1ORCID,Wu Hao2,Qu Yawei3,Xie Min4,Li Shu1ORCID,Zhuang Bingliang1ORCID,Li Mengmeng1ORCID,Kilifarska Natalya Andreeva5

Affiliation:

1. School of Atmospheric Sciences Nanjing University Nanjing China

2. Key Laboratory of Transportation Meteorology of China Meteorological Administration Nanjing Joint Institute for Atmospheric Sciences Nanjing China

3. College of Intelligent Science and Control Engineering Jinling Institute of Technology Nanjing China

4. School of Environment Nanjing Normal University Nanjing China

5. Climate Atmosphere and Waters Research Institute Bulgarian Academy of Sciences Sofia Bulgaria

Abstract

AbstractMethane (CH4) plays a crucial role in shaping terrestrial ecosystems due to its radiative effect and atmospheric photochemical reactions. In this study, we employed an enhanced regional climate‐chemistry‐ecosystem model (RegCM‐Chem‐YIBs) to comprehensively evaluate the impacts of both radiative and chemical effects of CH4 on terrestrial carbon fluxes across the East, South, and Southeast Asia (EA, SA, SEA) during the year 2010. Our findings showed that the radiative effects of CH4 yielded a positive influence on carbon fluxes. Specifically, the EA region experienced a significant increase in the gross primary production (GPP), reaching up to 0.515 Pg C Yr−1. In comparison, the SEA region exhibited a decrease in the net ecosystem exchange (NEE) of approximately −0.066 Pg C Yr−1. Further analysis revealed that alterations in radiation and vapor pressure deficit (VPD) were dominant drivers. Conversely, the chemical effects of CH4 lead to heightened regional surface ozone (O3) concentrations (2.704–3.115 ppb) and generate a negative response in carbon fluxes. Within the SEA region, GPP observed a decrease of up to −0.144 Pg C Yr−1, while NEE displayed a significant increase of 0.022 Pg C Yr−1. Taken together, the combined radiative and chemical effects of CH4 indicated a positive impact on regional carbon fluxes, with GPP increasing by 0.632 Pg C Yr−1 and NEE decreasing by −0.09 Pg C Yr−1. This holistic perspective is crucial for comprehending the intricate interactions linking climate change, atmospheric pollution, and the global carbon cycle.

Publisher

American Geophysical Union (AGU)

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