Before Förster. Initial excitation in photosynthetic light harvesting

Author:

Karki Khadga J.1234ORCID,Chen Junsheng1234,Sakurai Atsunori5678,Shi Qi1234,Gardiner Alastair T.910111213ORCID,Kühn Oliver14151617,Cogdell Richard J.910111213,Pullerits Tönu1234ORCID

Affiliation:

1. Chemical Physics and NanoLund

2. Lund University

3. 22100 Lund

4. Sweden

5. Institute of Industrial Science

6. The University of Tokyo

7. Tokyo 153-8505

8. Japan

9. Institute of Molecular, Cell and Systems Biology

10. College of Medical, Veterinary and Life Sciences

11. University of Glasgow

12. Glasgow G12 8QQ

13. UK

14. Institute of Physics

15. University of Rostock

16. 18059 Rostock

17. Germany

Abstract

Fluorescence detected double quantum coherence 2D spectroscopy reveals strong correlation between weakly coupled pigment pools directly after absorption of light before the Förster transfer regime sets in.

Funder

Vetenskapsrådet

Crafoordska Stiftelsen

Energimyndigheten

Knut och Alice Wallenbergs Stiftelse

Qatar National Research Fund

Horizon 2020 Framework Programme

China Sponsorship Council

U.S. Department of Energy

Japan Society for the Promotion of Science

Lundbeckfonden

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

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