Designed TiS2 nanosheets for efficient electrocatalytic reductive amination of biomass-derived furfurals

Author:

Zhang Man1,Xu Shaojun23ORCID,Boubeche Mebrouka4ORCID,Decarolis Donato23,Huang Yizhe1,Liu Biying1,Gibson Emma K.35ORCID,Li Xin1,Wang Yuchen1,Luo Huixia4ORCID,Catlow C. Richard A.236,Yan Kai1ORCID

Affiliation:

1. School of Environmental Science and Engineering, Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology, Sun Yat-sen University, Guangzhou 510275, China

2. School of Chemistry, Cardiff University, Main Building, Park Place, Cardiff, CF10 3AT, UK

3. UK Catalysis Hub, Research Complex at Harwell, Rutherford Appleton Laboratory, Harwell, OX11 0FA, UK

4. School of Materials Science and Engineering and Key Lab Polymer Composite & Functional Materials, Sun Yat-sen University, Guangzhou, 510275, China

5. School of Chemistry, Joseph Black Building, University of Glasgow, Glasgow G12 8QQ, UK

6. Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, UK

Abstract

Laminate TiS2 nanosheets were successfully constructed for the electrochemical synthesis of valuable primary amines using biomass-derived furfurals at mild temperature and pressure.

Funder

National Key Research and Development Program of China

National Ten Thousand Talent Program

Basic and Applied Basic Research Foundation of Guangdong Province

Scientific and Technological Planning Project of Guangzhou City

Engineering and Physical Sciences Research Council

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Environmental Chemistry

Reference67 articles.

1. Simple ruthenium-catalyzed reductive amination enables the synthesis of a broad range of primary amines

2. Reductive amination using cobalt-based nanoparticles for synthesis of amines

3. A general carbonyl alkylative amination for tertiary amine synthesis

4. A dual light-driven palladium catalyst: Breaking the barriers in carbonylation reactions

5. D. T.Smith , M. D.Delost , H.Qureshi and J. T.Njarðarson , Top 200 Pharmaceuticals by Retail Sales in 2020, https://njardarson.lab.arizona.edu/sites/njardarson.lab.arizona.edu/files/Top%20200%20Pharmaceuticals%20By%20Retail%20Sales%202020V3.pdf

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