Reshaping aromatic frameworks: expansion of aromatic system drives metallabenzenoids to metallapentalenes

Author:

Li Qian1ORCID,Fei Jiawei1,Ruan Kaidong1,Hua Yuhui2,Chen Dafa2ORCID,Luo Ming2,Xia Haiping12ORCID

Affiliation:

1. State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China

2. Shenzhen Grubbs Institute, Department of Chemistry, Southern University of Science and Technology, Shenzhen 518055, China

Abstract

The first skeletal rearrangement from one metallaaromatic framework to another.

Funder

National Natural Science Foundation of China

Guangdong Provincial Key Laboratory Of Catalysis

Science, Technology and Innovation Commission of Shenzhen Municipality

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

Reference75 articles.

1. J.Mortier , Arene Chemistry: Reaction Mechanisms and Methods for Aromatic Compounds , John Wiley & Sons Ltd , New Jersey , 2016

2. I.Fernandez , Aromaticity: Modern Computational Methods and Applications , Elsevier , 2021

3. The Energetics of Aromatic Hydrocarbons:  An Experimental Thermochemical Perspective

4. The Photochemical 1,3 Addition of Alcohols to Benzenes1

5. Impact of Excited-State Antiaromaticity Relief in a Fundamental Benzene Photoreaction Leading to Substituted Bicyclo[3.1.0]hexenes

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