Internal acidity scale and reactivity evaluation of chiral phosphoric acids with different 3,3′-substituents in Brønsted acid catalysis-Reference-Cited by-同舟云学术

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Internal acidity scale and reactivity evaluation of chiral phosphoric acids with different 3,3′-substituents in Brønsted acid catalysis

Published:2019 Issue:43 Volume:10 Page:10025-10034
ISSN:2041-6520
Container-title:Chemical Science
language:en
Short-container-title:Chem. Sci.

Author:

Rothermel Kerstin¹²³⁴,Melikian Maxime¹²³⁴,Hioe Johnny¹²³⁴,Greindl Julian¹²³⁴,Gramüller Johannes¹²³⁴,Žabka Matej¹²³⁴^ORCID,Sorgenfrei Nils¹²³⁴,Hausler Thomas¹²³⁴,Morana Fabio¹²³⁴,Gschwind Ruth M.¹²³⁴^ORCID

Affiliation:

1. Institut für Organische Chemie

2. Universität Regensburg

3. D-93053 Regensburg

4. Germany

Abstract

NMR H-bond analysis reveals an offset of internal and external acidities of catalysts and allows for a detailed reactivity analysis.

Funder

Deutsche Forschungsgemeinschaft

FP7 Ideas: European Research Council

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2019/SC/C9SC02342A

Reference78 articles.

1. Chiral Phosphoric Acids as Versatile Catalysts for Enantioselective Transformations

2. Complete Field Guide to Asymmetric BINOL-Phosphate Derived Brønsted Acid and Metal Catalysis: History and Classification by Mode of Activation; Brønsted Acidity, Hydrogen Bonding, Ion Pairing, and Metal Phosphates

3. Asymmetric Counteranion-Directed Catalysis: Concept, Definition, and Applications

4. Schiff Base Catalysts for the Asymmetric Strecker Reaction Identified and Optimized from Parallel Synthetic Libraries

5. A General Catalyst for the Asymmetric Strecker Reaction

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3. Highly acidic N-triflylphosphoramides as chiral Brønsted acid catalysts: the effect of weak hydrogen bonds and multiple acceptors on complex structures and aggregation;Chemical Science;2024

4. Enantioselective and Regiodivergent Synthesis of Dihydro-1,2-oxazines from Triene-Carbamates via Chiral Phosphoric Acid-Catalysis;Journal of the American Chemical Society;2023-11-27

5. A Route to Potent, Selective, and Biased Salvinorin Chemical Space;ACS Central Science;2023-07-12

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