Direct imaging of changes in aerosol particle viscosity upon hydration and chemical aging

Author:

Hosny N. A.1234ORCID,Fitzgerald C.1564,Vyšniauskas A.1234ORCID,Athanasiadis A.1234,Berkemeier T.78910ORCID,Uygur N.78910,Pöschl U.78910,Shiraiwa M.78910,Kalberer M.1564,Pope F. D.111213144ORCID,Kuimova M. K.1234

Affiliation:

1. Department of Chemistry

2. Imperial College London

3. London

4. UK

5. University of Cambridge

6. Cambridge

7. Multiphase Chemistry Department

8. Max Planck Institute for Chemistry

9. Mainz

10. Germany

11. School of Geography

12. Earth and Environmental Science

13. University of Birmingham

14. Edgbaston

Abstract

We report quantitative, real-time, online observations of microscopic viscosity changes in aerosol particles of atmospherically relevant composition, using fluorescence lifetime imaging (FLIM) of viscosity.

Funder

European Research Council

Engineering and Physical Sciences Research Council

Natural Environment Research Council

European Commission

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

Reference57 articles.

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2. Evolution of Organic Aerosols in the Atmosphere

3. Air Pollution-Related Illness: Effects of Particles

4. Acute Respiratory Effects of Particulate Air Pollution

5. Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene

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