Evolution of Organic Aerosols in the Atmosphere

Author:

Jimenez J. L.1,Canagaratna M. R.2,Donahue N. M.3,Prevot A. S. H.4,Zhang Q.56,Kroll J. H.27,DeCarlo P. F.148,Allan J. D.910,Coe H.9,Ng N. L.2,Aiken A. C.1,Docherty K. S.1,Ulbrich I. M.1,Grieshop A. P.3,Robinson A. L.3,Duplissy J.4,Smith J. D.11,Wilson K. R.11,Lanz V. A.412,Hueglin C.12,Sun Y. L.56,Tian J.5,Laaksonen A.1314,Raatikainen T.1314,Rautiainen J.13,Vaattovaara P.13,Ehn M.15,Kulmala M.1516,Tomlinson J. M.17,Collins D. R.17,Cubison M. J.1,Dunlea J.1,Huffman J. A.1,Onasch T. B.2,Alfarra M. R.4910,Williams P. I.910,Bower K.9,Kondo Y.18,Schneider J.19,Drewnick F.519,Borrmann S.1920,Weimer S.4521,Demerjian K.5,Salcedo D.22,Cottrell L.23,Griffin R.2324,Takami A.25,Miyoshi T.25,Hatakeyama S.25,Shimono A.26,Sun J. Y27,Zhang Y. M.27,Dzepina K.128,Kimmel J. R.1229,Sueper D.12,Jayne J. T.2,Herndon S. C.2,Trimborn A. M.2,Williams L. R.2,Wood E. C.2,Middlebrook A. M.2,Kolb C. E.2,Baltensperger U.4,Worsnop D. R.2131415,

Affiliation:

1. Cooperative Institute for Research in the Environmental Sciences and Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA.

2. Aerodyne Research, Billerica, MA, USA.

3. Center for Atmospheric Particle Studies, Carnegie Mellon University, Pittsburgh, PA, USA.

4. Laboratory of Atmospheric Chemistry, Paul Scherrer Institut, Villigen, Switzerland,

5. Atmospheric Sciences Research Center, State University of New York, Albany, NY, USA.

6. Department of Environmental Toxicology, University of California, Davis, CA, USA.

7. Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA.

8. Department of Atmospheric and Oceanic Science, University of Colorado, Boulder, CO, USA.

9. School of Earth, Atmospheric, and Environmental Science, University of Manchester, Oxford Road, Manchester, UK.

10. National Centre for Atmospheric Science, University of Manchester, Oxford Road, Manchester, UK.

11. Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA.

12. Empa, Laboratory for Air Pollution/Environmental Technology, Dübendorf, Switzerland.

13. Department of Physics, University of Kuopio, Kuopio, Finland.

14. Finnish Meteorological Institute, Helsinki, Finland.

15. Department of Physics, University of Helsinki, Helsinki, Finland.

16. Department of Applied Environmental Science, Stockholm University, Stockholm, Sweden.

17. Department of Atmospheric Sciences, Texas A&M University, College Station, TX, USA.

18. Research Center for Advanced Science and Technology, University of Tokyo, Tokyo, Japan.

19. Department of Particle Chemistry, Max Planck Institute for Chemistry, Mainz, Germany.

20. Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany.

21. Empa, Laboratory for Internal Combustion Engines, Dübendorf, Switzerland.

22. Centro de Investigaciones Quimicas, Universidad Autonoma del Estado de Morelos, Cuernavaca, Mexico.

23. Climate Change Research Center, University of New Hampshire, Durham, NH, USA.

24. Department of Civil and Environmental Engineering, Rice University, Houston, TX, USA.

25. Asian Environmental Research Group, National Institute for Environmental Studies, Tsukuba, Japan.

26. Sanyu Plant Service, Sagamihara, Japan.

27. Key Laboratory for Atmospheric Chemistry, Chinese Academy of Meteorological Sciences, Beijing, China.

28. Atmospheric Chemistry Division, National Center for Atmospheric Research, Boulder, CO, USA.

29. Tofwerk, Thun, Switzerland.

Abstract

Framework for Change Organic aerosols make up 20 to 90% of the particulate mass of the troposphere and are important factors in both climate and human heath. However, their sources and removal pathways are very uncertain, and their atmospheric evolution is poorly characterized. Jimenez et al. (p. 1525 ; see the Perspective by Andreae ) present an integrated framework of organic aerosol compositional evolution in the atmosphere, based on model results and field and laboratory data that simulate the dynamic aging behavior of organic aerosols. Particles become more oxidized, more hygroscopic, and less volatile with age, as they become oxygenated organic aerosols. These results should lead to better predictions of climate and air quality.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

Reference31 articles.

同舟云学术

1.学者识别学者识别

2.学术分析学术分析

3.人才评估人才评估

"同舟云学术"是以全球学者为主线,采集、加工和组织学术论文而形成的新型学术文献查询和分析系统,可以对全球学者进行文献检索和人才价值评估。用户可以通过关注某些学科领域的顶尖人物而持续追踪该领域的学科进展和研究前沿。经过近期的数据扩容,当前同舟云学术共收录了国内外主流学术期刊6万余种,收集的期刊论文及会议论文总量共计约1.5亿篇,并以每天添加12000余篇中外论文的速度递增。我们也可以为用户提供个性化、定制化的学者数据。欢迎来电咨询!咨询电话:010-8811{复制后删除}0370

www.globalauthorid.com

TOP

Copyright © 2019-2024 北京同舟云网络信息技术有限公司
京公网安备11010802033243号  京ICP备18003416号-3