Ultrafast delocalization of excitation in synthetic light-harvesting nanorings
Author:
Affiliation:
1. University of Oxford
2. Department of Physics
3. Clarendon Laboratory
4. Oxford
5. UK
6. Department of Chemistry
7. Chemistry Research Laboratory
8. School of Physics & Astronomy
9. University of Nottingham
10. Nottingham
Abstract
When light is absorbed by a nanoring consisting of 6–24 porphyrin units, the excitation delocalizes over the whole molecule within 200 fs. Highly symmetric nanorings exhibit thermally enhanced super-radiance.
Funder
Engineering and Physical Sciences Research Council
Publisher
Royal Society of Chemistry (RSC)
Subject
General Chemistry
Link
http://pubs.rsc.org/en/content/articlepdf/2015/SC/C4SC02424A
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