Observing long-range non-fullerene backbone ordering in real-space to improve the charge transport properties of organic solar cells

Author:

Bi Zhaozhao1234,Chen Kai56789,Gou Lu1011234,Guo Yuan1213141516,Zhou Xiaobo1234,Naveed Hafiz Bilal1234,Wang Jing1718192021,Zhu Qinglian1234,Yuan Jian1234,Zhao Chao1234,Zhou Ke1234,Chandrabose Sreelakshmi2289,Tang Zheng1718192021ORCID,Yi Yuanping1213141516ORCID,Hodgkiss Justin M.2289,Zhang Lei1011234,Ma Wei1234ORCID

Affiliation:

1. State Key Laboratory for Mechanical Behavior of Materials

2. Xi'an Jiaotong University

3. Xi'an 710049

4. China

5. Robinson Research Institute

6. Faculty of Engineering

7. Victoria University of Wellington

8. Wellington

9. New Zealand

10. MOE Key Laboratory for Nonequilibrium Synthesis and Modulation of Condensed Matter

11. School of Physics

12. Beijing National Laboratory for Molecular Science

13. Key Laboratory of Organic Solids

14. Institute of Chemistry

15. Chinese Academy of Sciences

16. 100190 Beijing

17. Center for Advanced Low-dimension Materials

18. State Key Laboratory for Modification of Chemical Fibers and Polymer Materials

19. College of Materials Science and Engineering

20. Donghua University

21. Shanghai 201620

22. MacDiarmid Institute for Advanced Materials and Nanotechnology

Abstract

The long-range backbone ordering in Y6 solid film is reported, which benefits charge generation and carrier lifetime in PM6:Y6 heterojunctions and drives the photovoltaic efficiency towards 16.8%.

Funder

National Natural Science Foundation of China

Ministry of Science and Technology of the People's Republic of China

Fundamental Research Funds for the Central Universities

China Postdoctoral Science Foundation

Higher Education Discipline Innovation Project

Marsden Fund

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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