Resolving charge transfer mechanisms in molecular tunnel junctions using dynamic charge transfer and static current–voltage measurements

Author:

Cao Liang1ORCID,Zhang Ziyu2,Thompson Damien3ORCID,Qi Dong-Chen4,Nijhui Christian A.5ORCID

Affiliation:

1. Anhui Key Laboratory of Low-Energy Quantum Materials and Devices, High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences, Hefei 230031, P. R. China

2. Department of Chemistry, National University of Singapore, 3 Science Drive, Singapore 117543, Singapore

3. Department of Physics, Bernal Institute, University of Limerick, Limerick V94 T9PX, Ireland

4. Centre for Materials Science, School of Chemistry and Physics, Queensland University of Technology, Brisbane, Queensland 4001, Australia

5. Hybrid Materials for Opto-Electronics Group, Department of Molecules and Materials, MESA+ Institute for Nanotechnology and Center for Brain-Inspired Nano Systems, Faculty of Science and Technology, University of Twente, P.O. Box 217, 7500 AE Enschede, The Netherlands

Abstract

Comparing the tunnelling decay coefficient β values obtained through the core-hole clock and junction J(V) measurements allow for the identification of the most likely orbital involved in charge transport measurements, derived from DFT calculations.

Funder

National Natural Science Foundation of China

National Research Foundation Singapore

Australian Research Council

Science Foundation Ireland

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,General Chemistry

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