Leveraging polymer architecture design with acylamino functionalization for electrolytes to enable highly durable lithium metal batteries

Author:

Zheng Jiayu1,Duan Lingyan1,Ma Hang2,An Qi1,Liu Qing1,Sun Yongjiang1,Zhao Genfu1,Tang Hanlin1,Li Yang1,Wang Shimin1,Xu Qijun1,Wang Lilian1,Guo Hong13ORCID

Affiliation:

1. International Joint Research Center for Advanced Energy Materials of Yunnan Province, School of Materials and Energy, Yunnan University, Kunming 650091, China

2. R & D Center, Yunnan Yuntianhua Co., Ltd, Kunming 650228, China

3. Southwest United Graduate School, Kunming 650091, China

Abstract

A novel polymer architecture design for GPEs is proposed via in situ copolymerization of VC and a new acylamino-crosslinker. This design enables accelerated Li+ transport and dual-reinforced stable interfaces, contributing to long-lifespan LMBs.

Funder

National Natural Science Foundation of China

Major Science and Technology Projects in Yunnan Province

Natural Science Foundation of Yunnan Province

Yunnan Provincial Department of Education

Publisher

Royal Society of Chemistry (RSC)

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