Effect of alkali metal addition on catalytic performance of Ag/ZrO<sub>2</sub>/SBA-16 catalyst for single-step conversion of ethanol to butadiene-Reference-Cited by-同舟云学术

Effect of alkali metal addition on catalytic performance of Ag/ZrO₂/SBA-16 catalyst for single-step conversion of ethanol to butadiene

Published:2023 Issue:4 Volume:13 Page:975-983
ISSN:2044-4753
Container-title:Catalysis Science & Technology
language:en
Short-container-title:Catal. Sci. Technol.

Author:

Winkelman Austin D.¹²^ORCID,Dagle Vanessa Lebarbier¹^ORCID,Lemmon Teresa L.¹,Kovarik Libor¹³^ORCID,Wang Yong¹²^ORCID,Dagle Robert A.¹

Affiliation:

1. Institute for Integrated Catalysis, Pacific Northwest National Laboratory, 902 Battelle Blvd., Richland, WA 99354, USA

2. Voiland School of Chemical Engineering and Bioengineering, Washington State University, Pullman, WA 99163, USA

3. Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, WA 99354, USA

Abstract

Alkali addition to a Ag/ZrO2/SBA-16 system for ethanol to butadiene affects a beneficial decrease in Lewis acid sites, mitigating ethanol dehydration. This results in remarkable butadiene selectivity and superior productivity over the lifetime study.

Funder

U.S. Department of Energy

Publisher

Royal Society of Chemistry (RSC)

Subject

Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2023/CY/D2CY01722A

Reference23 articles.

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4. Ethanol as a Renewable Building Block for Fuels and Chemicals

5. Annual Fuel Ethanol Production: U.S. and world Ethanol Production, 2020

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