Single-layer polymeric tetraoxa[8]circulene modified by s-block metals: toward stable spin qubits and novel superconductors

Author:

Begunovich Lyudmila V.1234,Kuklin Artem V.12345ORCID,Baryshnikov Gleb V.56789,Valiev Rashid R.101112413,Ågren Hans567814ORCID

Affiliation:

1. International Research Center of Spectroscopy and Quantum Chemistry (IRC SQC)

2. Siberian Federal University

3. Krasnoyarsk

4. Russia

5. Department of Physics and Astronomy

6. Uppsala University

7. SE-751 20 Uppsala

8. Sweden

9. Department of Chemistry and Nanomaterials Science

10. Research School of Chemistry & Applied Biomedical Sciences

11. National Research Tomsk Polytechnic University

12. Tomsk 634050

13. Department of Chemistry

14. College of Chemistry and Chemical Engineering

Abstract

Tetraoxa[8]circulene based 2D COFs doped with s-block metals possess metallic properties. Doping with Ca results in superconductivity and an open-shell singlet ground state composed of two doublets.

Funder

Russian Science Foundation

Stiftelsen Olle Engkvist Byggmästare

Ministry of Education and Science of Ukraine

Tomsk Polytechnic University

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science

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