A laser ablation resonance ionisation mass spectrometer (LA-RIMS) for the detection of isotope ratios of uranium at ultra-trace concentrations from solid particles and solutions

Author:

Strashnov Ilya1234ORCID,Izosimov Igor567,Gilmour Jamie D.8294,Denecke Melissa Anne10294ORCID,Almiral Jose11121314,Cannavan Andrew15161718,Chen Gang192021,Dissanayake Champa22232425,Doroshenko Iryna2627282930,Elghali Tibari3132333435,Enston Emma1234,Fernando Biyagamage Ruchika363725ORCID,Kasozi Gabriel38394041,Kelly Simon15161718,Maqsood Mohammed1234,Muhammad Syahidah Akmal42434445ORCID,Muryn Christopher1234,Pomerantsev Alexey L.464748ORCID,Singh Dileep Kumar4950515253,Smith Gareth1234,Taous Fouad3132333435ORCID,Webb Carole1234,Williamson David54554,Xu Zhenzhen192021,Yang Shuming192021,Zitek Andreas565758

Affiliation:

1. School of Chemistry

2. The University of Manchester

3. M13 9PL Manchester

4. UK

5. Obedinennyj institut adernyh issledovanij

6. Dubna

7. Russia

8. School of Earth Atmospheric and Environmental Science

9. Manchester

10. Dalton Nuclear Institute

11. Department of Chemistry and Biochemistry

12. Florida International University

13. OE116 Miami

14. USA 33156

15. International Atomic Energy Agency

16. Joint FAO/IAEA Division of Nuclear Techniques in Food & Agriculture

17. Vienna

18. Austria A-1400

19. Chinese Academy of Agricultural Sciences

20. Haidian District

21. China 100081

22. Sri Lanka Atomic Energy Board

23. Life Sciences Division

24. Colombo

25. Srilanka

26. Faculty of Physics

27. Experimental Physics Department

28. Taras Shevchenko National University of Kyiv

29. Kyiv

30. Ukraine

31. Centre National de l'Energie des Sciences et des Techniques Nucleaires

32. Laboratoire d'Analyses Structurales et Isotopiques (LASI)

33. Division Exploitation des Laboratoires

34. Rabat

35. Morocco

36. University of Peradeniya

37. Peradeniya

38. Department of Chemistry Kampala

39. Makerere University

40. Kampala

41. Uganda

42. School of Industrial Technology/Analytical Biochemistry Research Centre Minden

43. Universiti Sains Malaysia

44. Pulau Pinang

45. Malaysia

46. Semenov Institute of Chemical Physics RAS

47. Moscow

48. Russian Federation 119991

49. University of Delhi

50. Soil Microbial Ecology and Environmental Toxicology Laboratory

51. Department of Zoology

52. New Delhi

53. India

54. Oxford Instruments plc

55. Abingdon

56. University of Natural Resources and Life Sciences

57. Tulln

58. Austria A-3430

Abstract

A commercial MALDI mass spectrometer coupled with a tunable laser ionisation system can be used for the detection of uranium isotope ratios at trace levels.

Funder

Science and Technology Facilities Council

Publisher

Royal Society of Chemistry (RSC)

Subject

Spectroscopy,Analytical Chemistry

Reference34 articles.

1. T. B. Cochran , et al. , U.S. Nuclear Warhead Production , John Wiley Press , 1987

2. D. Holloway , The Soviet Union and the Arms Race , Cambridge University Press , 2nd edn, 1984

3. T. B. Cochran , Soviet Nuclear Weapons , Ballinger Pub Co , 1989

4. K. Janssens , et al. , Microscopic X-ray Fluorescence Analysis , Wiley , 2000

5. Invited Review Article: Recent developments in isotope-ratio mass spectrometry for geochemistry and cosmochemistry

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