Hybrid quantum-classical polarizability model for single molecule biosensing

Author:

Zossimova Ekaterina12ORCID,Fiedler Johannes3ORCID,Vollmer Frank1,Walter Michael245ORCID

Affiliation:

1. Department of Physics and Astronomy, Living Systems Institute, University of Exeter, EX4 4QD, Exeter, UK

2. Freiburg Center for Interactive Materials and Bioinspired Technologies (FIT), University of Freiburg, D-79110 Freiburg, Germany

3. Department of Physics and Technology, University of Bergen, Allégaten 55, 5007 Bergen, Norway

4. Cluster of Excellence livMatS @ FIT, Freiburg, Germany

5. Fraunhofer IWM, MikroTribologie Centrum μTC, Freiburg, Germany

Abstract

We present a 3-layer cavity model to calculate the polarizability of solvated molecules. By analogy, the different layers of our cavity model resemble the nested structure of a Matryoshka doll.

Funder

Engineering and Physical Sciences Research Council

H2020 Marie Skłodowska-Curie Actions

Deutsche Forschungsgemeinschaft

Publisher

Royal Society of Chemistry (RSC)

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