Catalyst-free, direct electrochemical synthesis of annulated medium-sized lactams through C–C bond cleavage

Author:

Xu Zhongnan12345,Huang Zhixing12345,Li Yueheng12345,Kuniyil Rositha6789,Zhang Chao12345,Ackermann Lutz6789ORCID,Ruan Zhixiong12345ORCID

Affiliation:

1. Key Laboratory of Molecular Target & Clinical Pharmacology and the State Key Laboratory of Respiratory Disease

2. School of Pharmaceutical Sciences & the Fifth Affiliated Hospital

3. Guangzhou Medical University

4. Guangzhou

5. P.R. China

6. Institut für Organische und Biomolekulare Chemie

7. Georg-August-Universität Göttingen

8. 37077 Göttingen

9. Germany

Abstract

Expanding ring under green electricity: The electrosynthetic approach enabled atom-economical synthesis of challenging medium-sized lactams through a unique remote amidyl migration under exceedingly mild, transition metal- and oxidant-free conditions.

Funder

National Natural Science Foundation of China

Guangzhou Municipal Science and Technology Project

Deutsche Forschungsgemeinschaft

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Environmental Chemistry

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