A MnOx enhanced atomically dispersed iron–nitrogen–carbon catalyst for the oxygen reduction reaction

Author:

Ding Shichao1ORCID,Lyu Zhaoyuan1,Sarnello Erik2,Xu Mingjie3ORCID,Fang Lingzhe2,Tian Hangyu1,Karcher Sam Ellery1,Li Tao24,Pan Xiaoqing3,McCloy John1ORCID,Ding Guodong5ORCID,Zhang Qiang5ORCID,Shi Qiurong1ORCID,Du Dan1ORCID,Li Jin-Cheng1ORCID,Zhang Xiao6ORCID,Lin Yuehe156ORCID

Affiliation:

1. School of Mechanical and Materials Engineering, Washington State University, Pullman, WA, 99164, USA

2. Department of Chemistry and Biochemistry, Northern Illinois University, DeKalb, IL, 60115, USA

3. Irvine Materials Research Institute (IMRI), Department of Materials Science and Engineering, University of California, Irvine, CA, 92697, USA

4. X-ray Science Division, Argonne National Laboratory, Lemont, IL, 60439, USA

5. Department of Chemistry, Washington State University, Pullman, Washington 99164, USA

6. School of Chemical Engineering and Bioengineering, Washington State University, USA

Abstract

A MnOx-assisted strategy is proposed to improve the oxygen reduction activity and stability of Fe–N–C single-atom catalysts (SACs) by regulating the electron structure and reducing the side effects of the Fenton reaction.

Funder

Washington State University

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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