Source apportionment and source-specific risk evaluation of potential toxic elements in oasis agricultural soils of Tarim River Basin

Abstract

AbstractAs rapidly developing area of intensive agriculture during the past half century, the oases in the source region of the Tarim River have encountered serious environmental challenges. Therefore, a comparative analysis of soil pollution characteristics and source-specific risks in different oases is an important measure to prevent and control soil pollution and provide guidance for extensive resource management in this area. In this study, the concentration of potential toxic elements (PTEs) was analyzed by collecting soil samples from the four oases in the source region of the Tarim River. The cumulative frequency curve method, pollution index method, positive matrix factorization (PMF) model, geographical detector method and health risk assessment model were used to analyze the pollution status and source-specific risk of potential toxic elements in different oases. The results showed that Cd was the most prominent PTE in the oasis agricultural soil in the source region of the Tarim River. Especially in Hotan Oasis, where 81.25% of the soil samples were moderately contaminated and 18.75% were highly contaminated with Cd. The PTEs in the Hotan Oasis corresponded to a moderate level of risk to the ecological environment, and the noncarcinogenic risk of soil PTEs in the four oases to local children exceeded the threshold (TH > 1), while the carcinogenic risk to local residents was acceptable (1E−06 < TCR < 1E−04). The research results suggested that the Hotan Oasis should be the key area for soil pollution control in the source region of the Tarim River, and agricultural activities and natural sources, industrial sources, and atmospheric dust fall are the priority sources that should be controlled in the Aksu Oasis, Kashgar Oasis and Yarkant River Oasis, respectively. The results of this study provide important decision-making support for the protection and management of regional agricultural soil and the environment.