1. Institute of Ecology, Friedrich Schiller University Jena, Dornburger Straβe 159, D-07743 Jena, Germany, Department of Oceanography, Florida State University, 255 Atomic Way, Tallahassee, Florida 32306, Institute of Radiochemistry, Forschungszentrum Dresden-Rossendorf, D-01314 Dresden, Germany, and The Rossendorf Beamline at ESRF, F-38043 Grenoble, France