1. Environmental Science Department, Institute of Environmental and Natural Sciences, Lancaster University, Lancaster, LA1 4YQ, U.K., Meteorological Service of Canada, Environment Canada, 4905 Dufferin Street, Downsview, Ontario M3H 5T4, Canada, Rothamsted Experimental Station, Harpenden, Hertfordshire AL5 2JQ, U.K., Department of Chemical Engineering & Applied Chemistry, University of Toronto, 200 College Street, Toronto, Ontario M5S 3E5, Canada