Abstract
Aerosol optical depth (AOD) measurements for 2017–2020 in urban Hohhot of the Mongolian plateau, a transition zone between the depopulated zone and East Asian urban agglomeration, were analyzed for the first time. Results show that annual AOD500 and Ångström exponent α440-675 were 0.36 ± 0.09 and 1.11 ± 0.16 (2017), 0.41 ± 0.12 and 0.90 ± 0.28 (2018), 0.38 ± 0.09 and 1.13 ± 0.24 (2019), 0.38 ± 0.12 and 1.17 ± 0.22 (2020), respectively, representing a slightly polluted level with a mixed type of coarse dust aerosol and a fine urban/industrial aerosol. Throughout the year, depopulated-zone continental air flows predominated in Hohhot (i.e., NW-quadrant wind), accounting for 82.12% (spring), 74.54% (summer), 63.61% (autumn), and 100% (winter). The clean and strong NW-quadrant air flows induced by the south movement of a Siberian anticyclone resulted in a low 500-nm AOD of 0.30 ± 0.29, 0.20 ± 0.15, 0.24 ± 0.29, and 0.13 ± 0.08 from spring to winter. Meanwhile, the local emissions from Hohhot city, as well as anthropogenic urban/industrial aerosols transported by southern and western air masses, originating from southern urban agglomeration and western industrial cities (Baotou, Wuhai, etc.), contributed to the highest aerosol loading, with significant transformation rates of the secondary aerosols Sulfate-Nitrate-Ammonium (SNA) of 47.45%, 57.39%, 49.88%, and 45.16–47.36% in PM2.5 for each season. The extinction fraction of fine aerosols under these anthropogenic trajectories can be as high as 80%, and the largest fine aerosol size was around 0.2–0.25 μm. Dust aerosols were suspending in urban Hohhot all year, although at different levels for different seasons, and the extinction fraction of dust aerosol during sandstorms was generally higher than 70%.
Funder
China Postdoctoral Science Foundation
the major science and technology project of Inner Mongolia Autonomous Region
National Natural Science Foundation of China
the Royal Society
Subject
Atmospheric Science,Environmental Science (miscellaneous)