Reactive Molecular Dynamics Study of Pollutant Formation Mechanism in Hydrogen/Ammonia/Methanol Ternary Carbon-Neutral Fuel Blend Combustion

Author:

Sun Jingyun1,Liu Qianqian1,Wang Yang12,Gu Mingyan1,Huang Xiangyong1

Affiliation:

1. School of Energy and Environment, Anhui University of Technology, Ma’anshan 243002, China

2. School of Materials Science and Engineering, Anhui University of Technology, Ma’anshan 243032, China

Abstract

Hydrogen, ammonia, and methanol are typical carbon-neutral fuels. Combustion characteristics and pollutant formation problems can be significantly improved by their blending. In this paper, reactive molecular dynamics were used to investigate the pollutant formation characteristics of hydrogen/ammonia/methanol blended fuel combustion and to analyze the mechanisms of CO, CO2, and NOX formation at different temperatures and blending ratios. It was found that heating can significantly increase blending and combustion efficiency, leading to more active oxidizing groups and thus inhibiting N2 production. Blended combustion pollutant formation was affected by coupling effects. NH3 depressed the rate of CO production when CH4O was greater than 30%, but the amount of CO and CO2 was mainly determined by CH4O. This is because CH4O provides more OH, H, and carbon atoms for CO and CO2 to collide efficiently. CH4O facilitates the combustion of NH3 by simplifying the reaction pathway, making it easier to form NOX.

Funder

National Natural Science Foundation of China

Natural Science Foundation of Anhui Province

University Synergy Innovation Program of Anhui Province

Funding for Postdoctoral Researchers’ ScientificResearch Activities in Anhui Province

Publisher

MDPI AG

Subject

Chemistry (miscellaneous),Analytical Chemistry,Organic Chemistry,Physical and Theoretical Chemistry,Molecular Medicine,Drug Discovery,Pharmaceutical Science

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