High sensitivity of semimetal photodetection via Bose–Einstein condensation

Author:

Wu Tuntan123ORCID,Qiu Qinxi13,Li Yongzhen13,Zhou Qiangguo13ORCID,Ma Wanli13,Li Jingbo13,Jiang Lin1,Zhou Wei1,Huang Zhiming12345

Affiliation:

1. State Key Laboratory of Infrared Physics Shanghai Institute of Technical Physics, Chinese Academy of Sciences Shanghai the People's Republic of China

2. Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences Hangzhou the People's Republic of China

3. University of Chinese Academy of Sciences Beijing the People's Republic of China

4. Institute of Optoelectronics, Fudan University Shanghai the People's Republic of China

5. Key Laboratory of Space Active Optical‐Electro Technology Chinese Academy of Sciences Shanghai the People's Republic of China

Abstract

AbstractThe discovery of semiconductor has witnessed remarkable strides toward high performance of photodetectors attributed to its excellent carrier properties. However, semimetal, owning to the high carrier concentration and low carrier mobility compared to those of semiconductor, is generally considered unsuitable for photodetection. Herein, we demonstrate an outstanding photodetection in a layered semimetal titanium diselenide (TiSe2) in Bose–Einstein condensation (BEC) state. High sensitivity of semimetal photodetector is realized in the range of visible, infrared and terahertz bands. The noise equivalent power (NEP) has threefold improvement at the visible and infrared wavebands, and significant decrease by one order of magnitude in the terahertz frequencies via BEC phenomenon, attributed to the electrical parameter variation after condensation. The best NEP value in the terahertz frequency is comparable to that of commercial Si photodetector. Our results show another recipe to fabricate high performance of photodetection via semimetal except for semiconductor and pave the way to exploit macroscopic quantum phenomena for optoelectronics.image

Funder

National Natural Science Foundation of China

Chinese Academy of Sciences

Publisher

Wiley

Subject

Materials Chemistry,Surfaces, Coatings and Films,Materials Science (miscellaneous),Electronic, Optical and Magnetic Materials

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