Influence of aluminum addition on structure, hardness, and oxidation resistance of Ta1−xAlxN thin films

Author:

Santos Jonh Yago Erikson1ORCID,Dias Iago Lemos1,Rezende Ronaldo Lima1,de Oliveira Givanilson Brito1,da Silva Neto Pedro Cardoso2,Mendes Fabiana Magalhães Teixeira3,Hübler Roberto4,Tentardini Eduardo Kirinus1

Affiliation:

1. Universidade Federal de Sergipe São Cristóvão SE Brazil

2. Universidade Federal da Bahia Salvador BA Brazil

3. Instituto Nacional de Tecnologia Rio de Janeiro RJ Brazil

4. Pontifícia Universidade Católica do Rio Grande do Sul Porto Alegre RS Brazil

Abstract

Ta1−xAlxN thin films with 5, 15, and 40 at.% Al addition were co‐deposited by reactive magnetron sputtering and characterized by Rutherford backscattering spectroscopy (RBS), grazing angle X‐ray diffraction (GAXRD), X‐ray photoelectron spectroscopy (XPS), scanning electron microscopy (SEM), nanohardness, and oxidation tests. GAXRD and XPS analyses showed, regardless of the % Al added, the non‐existence of ternary nitride Ta1−xAlxN, but always as individual binary nitrides, TaN and AlN. Sample TaAlN_15 obtained the highest hardness and H3/E2 values, possibly due to the AlN grains presence, which were efficient in distorting the TaN lattice. All samples failed oxidation tests at 873 K, showing that the Al addition was not efficient in improving this property for tantalum aluminum nitride thin films.

Funder

Coordenação de Aperfeiçoamento de Pessoal de Nível Superior

Universidade Federal de Sergipe

Conselho Nacional de Desenvolvimento Científico e Tecnológico

Fundação de Apoio à Pesquisa e à Inovação Tecnológica do Estado de Sergipe

Publisher

Wiley

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