Closed-Form Calculation of Coherent Anti-Stokes Raman and Stimulated Raman Scattering Spectral Profiles

Author:

Perkins P. E.1,Lewis J. W. L.1

Affiliation:

1. Arnold Engineering and Development Center, Tullahoma, Tennessee 37389

Abstract

The third-order susceptibility is expressed as a summation of interfering resonant terms, each involving the phenomenological linewidth of the transition. Correlations of the finite linewidth of the laser sources with |χ(3)|2 (coherent anti-Stokes Raman spectroscopy) and –χ” (stimulated Raman scattering) are performed and closed-form expressions for the theoretical profiles are obtained.

Publisher

SAGE Publications

Subject

Spectroscopy,Instrumentation

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