Rainforest Aerosols as Biogenic Nuclei of Clouds and Precipitation in the Amazon

Author:

Pöschl U.1,Martin S. T.2,Sinha B.1,Chen Q.2,Gunthe S. S.1,Huffman J. A.1,Borrmann S.1,Farmer D. K.3,Garland R. M.1,Helas G.1,Jimenez J. L.3,King S. M.2,Manzi A.4,Mikhailov E.15,Pauliquevis T.67,Petters M. D.89,Prenni A. J.8,Roldin P.10,Rose D.1,Schneider J.1,Su H.1,Zorn S. R.12,Artaxo P.6,Andreae M. O.1

Affiliation:

1. Max Planck Institute for Chemistry, 55128 Mainz, Germany.

2. School of Engineering and Applied Sciences and Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA 02138, USA.

3. Department of Chemistry and Biochemistry and Cooperative Institute for Research in Environmental Science, University of Colorado, Boulder, CO 80309, USA.

4. National Institute of Amazonian Research, 69060 Manaus, Brazil.

5. Atmospheric Physics Department, Institute of Physics, St. Petersburg State University, 198904 St. Petersburg, Russia.

6. Institute of Physics, University of São Paulo, 05508 São Paulo, Brazil.

7. Federal University of São Paulo, 04023 Diadema, Brazil.

8. Department of Atmospheric Science, Colorado State University, Fort Collins, CO 80523, USA.

9. Marine Earth and Atmospheric Science, North Carolina State University, Raleigh, NC 27695, USA.

10. Department of Physics, Lund University, 22100 Lund, Sweden.

Abstract

Clean or Dirty Aerosols strongly affect atmospheric properties and processes—including visibility, cloud formation, and radiative behavior. Knowing their effects in both clean and polluted air is necessary in order to understand their influence (see the Perspective by Baltensperger ). Clarke and Kapustin (p. 1488 ) examine vertical atmospheric profiles collected above the Pacific Ocean, where air quality is affected by the transport of polluted air from the west, and find significant regional enhancements in light scattering, aerosol mass, and aerosol number associated with combustion. Aerosol particle concentrations in this region can exceed values in clean, unperturbed regions by over an order of magnitude. Thus combustion affects hemispheric aerosol optical depth and the distribution of cloud condensation nuclei. Pöschl et al. (p. 1513 ) discuss the composition of aerosols above the Amazon Basin, in the pristine conditions of the rainy season. The aerosols in this region are derived mostly from gaseous biogenic precursors, plants, and microorganisms, and particle concentration is orders of magnitude lower than in polluted continental regions.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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