Atmospheric new particle formation from sulfuric acid and amines in a Chinese megacity

Author:

Yao Lei1ORCID,Garmash Olga2ORCID,Bianchi Federico32ORCID,Zheng Jun4ORCID,Yan Chao2,Kontkanen Jenni25ORCID,Junninen Heikki26ORCID,Mazon Stephany Buenrostro2ORCID,Ehn Mikael2ORCID,Paasonen Pauli2ORCID,Sipilä Mikko2,Wang Mingyi1,Wang Xinke1,Xiao Shan1,Chen Hangfei1,Lu Yiqun1ORCID,Zhang Bowen1,Wang Dongfang7,Fu Qingyan7,Geng Fuhai8,Li Li9,Wang Hongli9,Qiao Liping9ORCID,Yang Xin11011ORCID,Chen Jianmin11011ORCID,Kerminen Veli-Matti2,Petäjä Tuukka212ORCID,Worsnop Douglas R.213ORCID,Kulmala Markku32ORCID,Wang Lin1101113ORCID

Affiliation:

1. Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China.

2. Aerosol and Haze Laboratory, Beijing University of Chemical Technology, Beijing 100029, China.

3. Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland.

4. Department of Environmental Science and Analytical Chemistry (ACES) and Bolin Centre for Climate Research, Stockholm University, 10691 Stockholm, Sweden.

5. Laboratory of Environmental Physics, Institute of Physics, University of Tartu, Tartu 50411, Estonia.

6. Shanghai Environmental Monitoring Center, Shanghai 200030, China.

7. Shanghai Meteorology Bureau, Shanghai 200135, China.

8. Shanghai Academy of Environmental Sciences, Shanghai 200233, China.

9. Institute of Atmospheric Sciences, Fudan University, Shanghai 200433, China.

10. Collaborative Innovation Center of Climate Change, Nanjing 210023, China.

11. Joint International Research Laboratory of Atmospheric and Earth System Sciences (JirLATEST), Nanjing University, Nanjing 210023, China.

12. Aerodyne Research, Billerica, MA 01821, USA.

13. Shanghai Institute of Pollution Control and Ecological Security, Shanghai 200092, China.

Abstract

A puzzle of new particles Atmospheric particulates can be produced by emissions or form de novo. New particle formation usually occurs in relatively clean air. This is because preexisting particles in the atmosphere will scavenge the precursors of new particles and suppress their formation. However, observations in some heavily polluted megacities have revealed substantial rates of new particle formation despite the heavy loads of ambient aerosols. Yao et al. investigated new particle formation in Shanghai and describe the conditions that make this process possible. The findings will help inform policy decisions about how to reduce air pollution in these types of environments. Science , this issue p. 278

Funder

European Research Council

Swiss National Science Foundation

National Natural Science Foundation of China

Ministry of Science and Technology of China

Royal Society-Newton Advanced Fellowship

European Union’s Horizon 2020 research and innovation programme

Cyrus Tang Foundation

the Academy of Finland Centre of Excellence program

the Academy of Finland via Academy Professorship

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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