Controlling the Morphology of Amorphous Solid Water

Author:

Stevenson K. P.1,Kimmel Greg A.1,Dohnálek Z.1,Smith R. Scott1,Kay Bruce D.1

Affiliation:

1. Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Post Office Box 999, Mail Stop K8-88, Richland, WA 99352, USA.

Abstract

The morphology of amorphous solid water grown by vapor deposition was found to depend strongly on the angular distribution of the water molecules incident from the gas phase. Systematic variation of the incident angle during deposition using a collimated beam of water led to the growth of nonporous to highly porous amorphous solid water. The physical and chemical properties of amorphous solid water are of interest because of its presence in astrophysical environments. The ability to control its properties in the laboratory may shed light on some of the outstanding conflicts related to this important material.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

Reference33 articles.

1. Structural Transitions in Amorphous Water Ice and Astrophysical Implications

2. Smoluchowski R., ibid. 201, 809 (1978).

3. A. G. G. M. Tielens and L. J. Allamandola in Composition Structure and Chemistry of Interstellar Dust J. D. J. Hollenbach and H. A. Thronson Eds. (Reidel Dordrecht Netherlands 1986) pp. 397–469.

4. Speedy R. J., Debenedetti P. G., Smith R. S., Huang C., Kay B. D., J. Chem. Phys. 105, 240 (1996).

5. P. G. Debenedetti Metastable Liquids: Concepts and Principles (Princeton Univ. Press Princeton NJ 1996).

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