Visualizing the atomic-scale origin of metallic behavior in Kondo insulators

Author:

Pirie Harris12ORCID,Mascot Eric3ORCID,Matt Christian E.1ORCID,Liu Yu1ORCID,Chen Pengcheng1ORCID,Hamidian M. H.1ORCID,Saha Shanta4ORCID,Wang Xiangfeng4,Paglione Johnpierre4ORCID,Luke Graeme5ORCID,Goldhaber-Gordon David67ORCID,Hirjibehedin Cyrus F.8910ORCID,Davis J. C. Séamus2111213ORCID,Morr Dirk K.3ORCID,Hoffman Jennifer E.1ORCID

Affiliation:

1. Department of Physics, Harvard University, Cambridge, MA 02138, USA.

2. Clarendon Laboratory, University of Oxford, Oxford OX1 3PU, UK.

3. Department of Physics, University of Illinois at Chicago, Chicago, IL 60607, USA.

4. Maryland Quantum Materials Center, Department of Physics, University of Maryland, College Park, MD 20742, USA.

5. Department of Physics and Astronomy, McMaster University, Hamilton, ON L8S 4M1, Canada.

6. Department of Physics, Stanford University, Stanford, CA 94305, USA.

7. Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

8. London Centre for Nanotechnology, University College London (UCL), London WC1H 0AH, UK.

9. Department of Physics and Astronomy, UCL, London WC1E 6BT, UK

10. Department of Chemistry, UCL, London WC1H 0AJ, UK.

11. Department of Physics, University College Cork, Cork T12 R5C, Ireland.

12. Laboratory of Atomic and Solid State Physics, Department of Physics, Cornell University, Ithaca, NY 14850, USA.

13. Max Planck Institute for Chemical Physics of Solids, D-01187 Dresden, Germany.

Abstract

A Kondo lattice is often electrically insulating at low temperatures. However, several recent experiments have detected signatures of bulk metallicity within this Kondo insulating phase. In this study, we visualized the real-space charge landscape within a Kondo lattice with atomic resolution using a scanning tunneling microscope. We discovered nanometer-scale puddles of metallic conduction electrons centered around uranium-site substitutions in the heavy-fermion compound uranium ruthenium silicide (URu 2 Si 2 ) and around samarium-site defects in the topological Kondo insulator samarium hexaboride (SmB 6 ). These defects disturbed the Kondo screening cloud, leaving behind a fingerprint of the metallic parent state. Our results suggest that the three-dimensional quantum oscillations measured in SmB 6 arise from Kondo-lattice defects, although we cannot exclude other explanations. Our imaging technique could enable the development of atomic-scale charge sensors using heavy-fermion probes.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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