STUDY OF CATALYSTS BASED ON MESOPOROUS ALUMINOSILICATE IN THE DEAROMATIZATION PROCESS OF A MODEL MIXTURE: PHYSICO-CHEMICAL CHARACTERISTICS AND CATALYTIC ACTIVITY

Author:

Abdrassilova A.1ORCID,Vassilina G.1ORCID,Abdildina K.1ORCID,Kanapiyeva F.1ORCID

Affiliation:

1. al-Farabi Kazakh National university

Abstract

The limitation on the content of aromatic hydrocarbons and sulfur is associated with environmental requirements according to Euro-5 standards. Upon combustion, these substances release highly toxic compounds into the atmosphere, adversely affecting human health and the surrounding environment. Additionally, a high concentration of aromatic hydrocarbons in diesel fuel significantly degrades its quality, leading to soot formation and reducing its cetane number. According to Euro-5 standards, the content of polycyclic aromatic hydrocarbons and sulfur compounds should not exceed 8% and 10 mg/kg, respectively. To address the challenge of producing high-quality diesel fuels, the hydrotreatment process is employed in the presence of heterogeneous catalysts.The article presents the synthesis of mesoporous aluminosilicates and bifunctional catalysts based on them to study the activity of the hydrotreatment process for a model mixture. The obtained samples were investigated using various physico-chemical methods such as SEM, low-temperature nitrogen adsorption/desorption, XRD, and FT-IR. It was established that the Ni/MAS-H-bentonite and Mo/MAS-H-bentonite catalysts exhibit high activity and selectivity in the hydrotreatment process under optimal conditions (240°C, 3 MPa, and 0.5 h-1).

Publisher

Shakarim University

Reference25 articles.

1. Yun G. The synthesis and mechanistic studies of a highly active nickel phosphide catalyst for naphthalene hydrodearomatization / G. Yun, Q. Guan, W. Li // RSC Advances. – 2017. – V. 7. – P. 8677-8687.

2. Regulation (EC) No 715/2007 of the European Parliament and of the Council of 20 June 2007 on type approval of motor vehicles with respect to emissions from light passenger and commercial vehicles (Euro 5 and Euro 6) and on access to vehicle repair and maintenance information. – 2007 – V. 030 (13) – P.284-299.

3. Effects of Fuel Sulfur Content and Diesel Oxidation Catalyst on PM Emitted from Light-Duty Diesel Engine / Zhao H., Ge Yu., Wang X. and etc. // Energy Fuels. – 2010. – V. 24. – P. 985-991.

4. Walendziewski J. Hydrodearomatization of diesel fuels using zeolite based catalysts. / J. Walendziewski, J. Grzechowiak, B. Pniak // Erdoel Erdgas Kohle. – 2000. – V. 116. – P. 297-303.

5. Al2O3-TiO2/ Al2O3-TiO2-SiO2 composite-supported bimetallic Pt-Pd catalysts for the hydrodearomatization and hydrodesulfurization of diesel fuel / W. Guofu, D. Aijun, Z. Zhen and etc. // Energy and Fuels. – 2009. – V. 23. – P. 81-85.

同舟云学术

1.学者识别学者识别

2.学术分析学术分析

3.人才评估人才评估

"同舟云学术"是以全球学者为主线,采集、加工和组织学术论文而形成的新型学术文献查询和分析系统,可以对全球学者进行文献检索和人才价值评估。用户可以通过关注某些学科领域的顶尖人物而持续追踪该领域的学科进展和研究前沿。经过近期的数据扩容,当前同舟云学术共收录了国内外主流学术期刊6万余种,收集的期刊论文及会议论文总量共计约1.5亿篇,并以每天添加12000余篇中外论文的速度递增。我们也可以为用户提供个性化、定制化的学者数据。欢迎来电咨询!咨询电话:010-8811{复制后删除}0370

www.globalauthorid.com

TOP

Copyright © 2019-2024 北京同舟云网络信息技术有限公司
京公网安备11010802033243号  京ICP备18003416号-3