Abstract
Abstract
In the progress of nanoengineering of noble metals, the extreme nonlinear optics within nanometric volumes is of great research interest in recent years. In particular, plasmonic nanostructures offer unique route for enhancing high-order harmonic generation and other nonlinear optical progress. Here, we report that strong third harmonic emission in zinc oxide (ZnO) microbelts (MBs) via a strong localization of electromagnetic field caused by localized surface plasmon resonances. In MB/Au-nanoparticles composite, it was demonstrated that the intensity of third-harmonic generation (THG) was enhanced by a factor of five compared to bare MB. Additionally, the polarization characteristics of THG in the same system were illustrated in detail. With respect to the bare MB, the polarization degree of THG was improved significantly. The nonlinear polarization features can be attributed to the crystal structure and the ensemble of anisotropic plasmonic hot spots on the surface of Au nanoparticles. Finally, intrinsic enhancement process of THG was explored comprehensively by finite difference time domain method. The simulation results are consistent with our experimental observation.
Funder
Science and Technology Program of Guangzhou
Joint Founds of the X LAB, The Second Academy of CASIC
National Natural Science Foundation of China
Subject
Surfaces, Coatings and Films,Acoustics and Ultrasonics,Condensed Matter Physics,Electronic, Optical and Magnetic Materials
Cited by
2 articles.
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