Tunable three-dimensional architecture of nematic disclination lines

Author:

Modin Alvin1ORCID,Ash Biswarup2,Ishimoto Kelsey1ORCID,Leheny Robert L.1ORCID,Serra Francesca13ORCID,Aharoni Hillel2ORCID

Affiliation:

1. Department of Physics and Astronomy, Johns Hopkins University, Baltimore, MD 21218

2. Department of Physics of Complex Systems, Weizmann Institute of Science, Rehovot 76100, Israel

3. Department of Physics, Chemistry, and Pharmacy, University of Southern Denmark, Odense DK-5230, Denmark

Abstract

Disclination lines play a key role in many physical processes, from the fracture of materials to the formation of the early universe. Achieving versatile control over disclinations is key to developing novel electro-optical devices, programmable origami, directed colloidal assembly, and controlling active matter. Here, we introduce a theoretical framework to tailor three-dimensional disclination architecture in nematic liquid crystals experimentally. We produce quantitative predictions for the connectivity and shape of disclination lines found in nematics confined between two thinly spaced glass substrates with strong patterned planar anchoring. By drawing an analogy between nematic liquid crystals and magnetostatics, we find that i) disclination lines connect defects with the same topological charge on opposite surfaces and ii) disclination lines are attracted to regions of the highest twist. Using polarized light to pattern the in-plane alignment of liquid crystal molecules, we test these predictions experimentally and identify critical parameters that tune the disclination lines’ curvature. We verify our predictions with computer simulations and find nondimensional parameters enabling us to match experiments and simulations at different length scales. Our work provides a powerful method to understand and practically control defect lines in nematic liquid crystals.

Funder

United States - Israel Binational Science Foundation

National Science Foundation

Publisher

Proceedings of the National Academy of Sciences

Subject

Multidisciplinary

Cited by 6 articles. 订阅此论文施引文献 订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献

1. Escape into the third dimension in cholesteric liquid crystals;New Journal of Physics;2024-06-01

2. A tensor density measure of topological charge in three-dimensional nematic phases;Proceedings of the Royal Society A: Mathematical, Physical and Engineering Sciences;2024-05

3. Frank-Read Mechanism in Nematic Liquid Crystals;Physical Review X;2024-03-11

4. Spatial Photo‐Patterning of Nematic Liquid Crystal Pretilt and its Application in Fabricating Flat Gradient‐Index Lenses;Advanced Materials;2024-03-07

5. Tunable three-dimensional architecture of nematic disclination lines;Proceedings of the National Academy of Sciences;2023-06-26

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