Identification of multiple natural and anthropogenic sources of dust in snow from Zhongshan Station to Dome A, East Antarctica

Abstract

ABSTRACTThe stable oxygen isotope composition, major ions and isotopic compositions of strontium (Sr), neodymium (Nd) and lead (Pb) in insoluble dust from recent surface snow samples along the transect from the Zhongshan and Progress stations (located on the Amery Ice Shelf, East Antarctica) to Dome A (Summit, Antarctica) were analysed. No previous isotopic fingerprinting studies have been conducted for this transect. These data were used to document the dust provenances in Antarctica along the transect up to the highest site, Dome A, for the first time. The insoluble dust in snow samples along the coast displays an overall crust-line isotopic signature that is characterised by highly radiogenic 87Sr/86Sr values and less radiogenic 143Nd/144Nd values. These signatures are comparable with those of samples collected near the ice-free areas of the Zhongshan and Progress stations. Spatial differences are statistically significant along the transect, and the Sr, Nd and Pb isotope components in insoluble dust from two continuous snow samples at Dome A exhibit marked differences, indicating that additional dust reaches the East Antarctic Plateau. The isotopic characteristics of insoluble dust from this transect indicate that the long-distance natural dust and anthropogenic pollutants in these samples primarily originate from Australia.