Spatial Aberrations in High-Order Harmonic Generation

Author:

Plach Marius1ORCID,Vismarra Federico123ORCID,Appi Elisa1ORCID,Poulain Vénus1ORCID,Peschel Jasper1ORCID,Smorenburg Peter4,O’Dwyer David P.4,Edward Stephen4,Tao Yin4,Borrego-Varillas Rocío3ORCID,Nisoli Mauro3ORCID,Arnold Cord L.1ORCID,L’Huillier Anne1,Eng-Johnsson Per1ORCID

Affiliation:

1. Department of Physics, Lund University, P.O. Box 118, 22100 Lund, Sweden.

2. Department of Physics, Politecnico di Milano, 20133 Milano, Italy.

3. Institute for Photonics and Nanotechnologies, IFN-CNR, 20133 Milano, Italy.

4. ASML Research, ASML Netherlands B.V., 5504 DR, Veldhoven, Netherlands.

Abstract

We investigate the spatial characteristics of high-order harmonic radiation generated in argon and observe cross-like patterns in the far field. An analytical model describing harmonics from an astigmatic driving beam reveals that these patterns result from the order and generation position-dependent divergence of harmonics. Even small amounts of driving field astigmatism may result in cross-like patterns, coming from the superposition of individual harmonics with spatial profiles elongated in different directions. By correcting the aberrations using a deformable mirror, we show that fine-tuning the driving wavefront is essential for optimal spatial quality of the harmonics.

Funder

Vetenskapsrådet

H2020 European Research Council

Knut och Alice Wallenbergs Stiftelse

Wallenberg Center for Quantum Technology, Chalmers University of Technology

Helmholtz-Lund International Graduate School

Publisher

American Association for the Advancement of Science (AAAS)

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