Ultrasensitive Frequency Shifting of Dielectric Mie Resonance near Metallic Substrate

Author:

Liu Chuanbao1,Wang Changxin2,Chen Junhong1,Su Yanjing2,Qiao Lijie2,Zhou Ji3,Bai Yang2

Affiliation:

1. School of Materials Science and Engineering, University of Science and Technology Beijing, Beijing 100083, China

2. Beijing Advanced Innovation Center for Materials Genome Engineering, Institute for Advanced Materials and Technology, University of Science and Technology Beijing, Beijing 100083, China

3. State Key Laboratory of New Ceramics and Fine Processing, Tsinghua University, Beijing 100084, China

Abstract

Dielectric resonators on metallic surface can enhance far-field scattering and boost near-field response having promising applications in nonlinear optics and reflection-type devices. However, the dependence of gap size between dielectric resonator and metallic surface on Mie resonant frequency is complex and desires a comprehensive physical interpretation. Here, we systematically study the effect of metallic substrate on the magnetic dipole (MD) resonant frequency at X-band by placing a high permittivity CaTiO 3 ceramic block on metallic substrate and regulating their gap size. The simulated and experimental results show that there are two physical mechanisms to codetermine the metallic substrate-induced MD frequency. The greatly enhanced electric field pair in the gap and the coupling of MD resonance with its mirror image are decisive for small and large gaps, respectively, making the MD resonant frequency present an exponential blue shift first and then a slight red shift with increasing gap size. Further, we use the two mechanisms to explain different frequency shifting properties of ceramic sphere near metallic substrate. Finally, taking advantage of the sharp frequency shifting to small gaps, the ceramic block is demonstrated to accurately estimate the thickness or permittivity of thin film on metallic substrate through a governing equation derived from the method of symbolic regression. We believe that our study will help to understand the resonant frequency shifting for dielectric particle near metallic substrate and give some prototypes of ultrasensitive detectors.

Funder

National Postdoctoral Program for Innovative Talents

Beijing Municipal Science and Technology Project

National Natural Science Foundation of China

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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